Revealing hidden defects through stored energy measurements of radiation damage
| Autor: | Charles A. Hirst, Fredric Granberg, Boopathy Kombaiah, Penghui Cao, Scott Middlemas, R. Scott Kemp, Ju Li, Kai Nordlund, Michael P. Short |
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| Přispěvatelé: | Department of Physics, Faculty of Science |
| Rok vydání: | 2022 |
| Předmět: | |
| Zdroj: | Science advances, vol 8, iss 31 |
| ISSN: | 2375-2548 |
| Popis: | With full knowledge of a material's atomistic structure, it is possible to predict any macroscopic property of interest. In practice, this is hindered by limitations of the chosen characterisation techniques. For example, electron microscopy is unable to detect the smallest and most numerous defects in irradiated materials. Instead of spatial characterisation, we propose to detect and quantify defects through their excess energy. Differential scanning calorimetry (DSC) of irradiated Ti measures defect densities 5 times greater than those determined using transmission electron microscopy (TEM). Our experiments also reveal two energetically-distinct processes where the established annealing model predicts one. Molecular dynamics (MD) simulations discover the defects responsible and inform a new mechanism for the recovery of irradiation-induced defects. The combination of annealing experiments and simulations can reveal defects hidden to other characterisation techniques, and has the potential to uncover new mechanisms behind the evolution of defects in materials. Comment: main: 17 pages and 6 figures, supplemental: 25 pages and 16 figures |
| Databáze: | OpenAIRE |
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