Two-phase dielectric polar structures in 0.1NBT-0.6ST-0.3PT solid solutions
| Autor: | Eriks Birks, Š. Svirskas, Vladimir V. Shvartsman, J. Banys, T. Ostapchuk, M. Dunce, Stanislav Kamba, Doru C. Lupascu, R. Ignatans |
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| Jazyk: | angličtina |
| Rok vydání: | 2018 |
| Předmět: |
010302 applied physics
Phase transition Materials science Polymers and Plastics Condensed matter physics Metals and Alloys 02 engineering and technology Dielectric 021001 nanoscience & nanotechnology Polarization (waves) 01 natural sciences Ferroelectricity Electronic Optical and Magnetic Materials Condensed Matter::Materials Science Piezoresponse force microscopy Phase (matter) 0103 physical sciences Ceramics and Composites Relaxation (physics) 0210 nano-technology Solid solution Bauwissenschaften |
| Popis: | In this work we address the peculiarities of the macroscopic responses in ternary 0.1Na0·5Bi0·5TiO3-0.6SrTiO3-0.3PbTiO3 (0.1NBT-0.6ST-0.3PT) solid solutions. These solid solutions exhibit a spontaneous first order relaxor to normal ferroelectric phase transition. The phase transition is accompanied by a broad dielectric relaxation which expands over 10 orders of magnitude in frequency just above the phase transition temperature. The temperature dependence of polarization shows that non-zero net polarization persists above the phase transition temperature. Below the phase transition temperature, it is not possible to describe the temperature dependence of polarization with a power law function which is valid in normal ferroelectrics. The piezoresponse force microscopy studies reveal that 0.1NBT-0.6ST-0.3PT solids solutions display several local polarization patterns which arise due to the bimodal distribution of grains in the ceramics. We associate the peculiar macroscopic responses to these complex polar structures and their different temperature behaviours. |
| Databáze: | OpenAIRE |
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