Spatially resolved electronic structure of twisted graphene

Autor: Qirong Yao, Paul Leonardus de Boeij, Kai Sotthewes, Shengjun Yuan, Pantelis Bampoulis, Guus J. Slotman, Lijie Zhang, Sebastiaan Haartsen, Henricus J.W. Zandvliet, Arie van Houselt, Rik van Bremen
Přispěvatelé: Physics of Interfaces and Nanomaterials, Physics of Fluids, Advanced Technology
Jazyk: angličtina
Rok vydání: 2017
Předmět:
Zdroj: Physical review B: Covering condensed matter and materials physics, 95(24):245116. American Institute of Physics
Physical Review B, 95, pp. 1-6
MESA+ Meeting 2017
Physical Review B, 95, 1-6
ISSN: 2469-9950
Popis: We have used scanning tunneling microscopy and spectroscopy to resolve the spatial variation of the density of states of twisted graphene layers on top of a highly oriented pyrolytic graphite substrate. Owing to the twist a moire pattern develops with a periodicity that is substantially larger than the periodicity of a single layer graphene. The twisted graphene layer has electronic properties that are distinctly different from that of a single layer graphene due to the nonzero interlayer coupling. For small twist angles (about 1-3.5 degree) the integrated differential conductivity spectrum exhibits two well-defined Van Hove singularities. Spatial maps of the differential conductivity that are recorded at energies near the Fermi level exhibit a honeycomb structure that is comprised of two inequivalent hexagonal sub-lattices. For energies |E-E_F|>0.3 eV the hexagonal structure in the differential conductivity maps vanishes. We have performed tight-binding calculations of the twisted graphene system using the propagation method, in which a third graphene layer is added to mimic the substrate. This third layer lowers the symmetry and explains the development of the two hexagonal sub-lattices in the moire pattern. Our experimental results are in excellent agreement with the tight-binding calculations.
To appear in Phys. Rev. B
Databáze: OpenAIRE