Spatially Controlled Fabrication of Surface-Enhanced Raman Scattering Hot Spots through Photoinduced Dewetting of Silver Thin Films
Autor: | Han-Kyu Choi, Sang-Min Park, Jeeyoon Jeong, Hankyul Lee, Gyu Jin Yeon, Dai-Sik Kim, Zee Hwan Kim |
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Rok vydání: | 2022 |
Předmět: | |
Zdroj: | The Journal of Physical Chemistry Letters. 13:2969-2975 |
ISSN: | 1948-7185 |
DOI: | 10.1021/acs.jpclett.2c00403 |
Popis: | A well-designed narrow gap between noble metal nanostructures plays a prominent role in surface-enhanced Raman scattering (SERS) to concentrate electromagnetic fields at the local point, called a "hot spot". However, SERS-active substrate fabrication remains a substantial hurdle due to the high process cost and the difficulty of engineering efficient plasmonic hot spots at the target area. In this study, we demonstrate a simple photolithographic method for generating ultrasensitive SERS hot spots at desired positions. The solid-state dewetting of a Ag thin film (thickness of ∼10 nm) using a continuous-wave laser (∼1 MW/cm |
Databáze: | OpenAIRE |
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