Carbon Dioxide-Free Hydrogen Production with Integrated Hydrogen Separation and Storage
| Autor: | Holger Jorschick, Regina Palkovits, Marta Helmin, Stefan Dürr, Andreas Bösmann, Peter Wasserscheid, Michael Müller |
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| Rok vydání: | 2016 |
| Předmět: |
General Chemical Engineering
Inorganic chemistry 02 engineering and technology Hydrogen purifier Steam reforming Hydrogen storage Hydrogen economy 0502 economics and business Environmental Chemistry General Materials Science 050207 economics Compressed hydrogen Hydrogen production Cryo-adsorption Chemistry business.industry 05 social sciences Carbon Dioxide 021001 nanoscience & nanotechnology Oxygen Hydrogen carrier General Energy Hydrogenation 0210 nano-technology business Hydrogen |
| Zdroj: | ChemSusChem. 10:42-47 |
| ISSN: | 1864-5631 |
| DOI: | 10.1002/cssc.201600435 |
| Popis: | An integration of CO2 -free hydrogen generation through methane decomposition coupled with hydrogen/methane separation and chemical hydrogen storage through liquid organic hydrogen carrier (LOHC) systems is demonstrated. A potential, very interesting application is the upgrading of stranded gas, for example, gas from a remote gas field or associated gas from off-shore oil drilling. Stranded gas can be effectively converted in a catalytic process by methane decomposition into solid carbon and a hydrogen/methane mixture that can be directly fed to a hydrogenation unit to load a LOHC with hydrogen. This allows for a straight-forward separation of hydrogen from CH4 and conversion of hydrogen to a hydrogen-rich LOHC material. Both, the hydrogen-rich LOHC material and the generated carbon on metal can easily be transported to destinations of further industrial use by established transport systems, like ships or trucks. |
| Databáze: | OpenAIRE |
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