Regional Atmospheric Budgets of Reduced Nitrogen Over the British Isles Assessed Using a Multi-Layer Atmospheric Transport Model

Autor: Y. de Kluizenaar, N. Fournier, Ulrike Dragosits, Y. S. Tang, Mark A. Sutton
Přispěvatelé: TNO Kwaliteit van Leven
Rok vydání: 2005
Předmět:
Nitrogen balance
Atmospheric chemistry
Atmospheric transport
British Isles
Air pollution
medicine.disease_cause
Atmospheric sciences
ammonia
Troposphere
Urban Development
Built Environment
comparative study
Water Science and Technology
Mathematical models
Atmospheric composition
atmospheric pollution
Ecological Modeling
article
Pollution
Nitrogen
transport kinetics
nitrogen deposition
Europe
Deposition (aerosol physics)
England
Eastern Hemisphere
politics
Geosciences
Ammonium
budget
Environmental Engineering
Meteorology
Western Europe
chemistry.chemical_element
reduction
Northern Ireland
concentration process
environmental impact
Atmosphere
medicine
Environmental Chemistry
Deposition
Wales
model
Atmospheric budget
atmospheric deposition
World
United Kingdom
Scotland
chemistry
validation process
Eurasia
Environmental science
Ireland
Zdroj: Water, Air, and Soil Pollution, 1-4, 162, 331-351
ISSN: 1573-2932
0049-6979
DOI: 10.1007/s11270-005-7249-0
Popis: Atmospheric budgets of reduced nitrogen for the major political regions of the British Isles are investigated with a multi-layer atmospheric transport model. The model is validated against measurements of NH3 concentration and is developed to provide atmospheric budgets for defined subdomains of the British Isles. The study shows that NH3 emissions, transport and deposition in a specific region can have profound effects on the composition of the atmosphere over other regions. An important feature is the high export of reduced nitrogen from Republic of Ireland and Northern Ireland to England and Scotland. England is also a net exporter of reduced nitrogen. By contrast, Scotland and Wales are approximately "ammonia neutral" as import of reduced nitrogen roughly balances export. Overall, only 7% of reduced nitrogen in the British Isles is derived from non-British Isles sources (29 kt N yr-1), compared with emissions of 387 kt N yr-1. Most of the reduced nitrogen is deposited in the British Isles (64%), while 36% is exported (148 kt N yr-1). © Springer 2005.
Databáze: OpenAIRE