Detailed MCNP simulations of gamma-ray spectroscopy measurements with calibration blocks for uranium mining applications

Autor: Jean-Luc Ma, P. G. Allinei, Bertrand Perot, P. Chaussonnet, T. Marchais, H. Toubon, Cedric Carasco
Přispěvatelé: CEA-Direction des Energies (ex-Direction de l'Energie Nucléaire) (CEA-DES (ex-DEN)), Commissariat à l'énergie atomique et aux énergies alternatives (CEA), amplexor, amplexor, Groupe AREVA
Jazyk: angličtina
Rok vydání: 2017
Předmět:
[PHYS.NUCL] Physics [physics]/Nuclear Theory [nucl-th]
Nuclear and High Energy Physics
Nuclear measurements
Materials science
[PHYS.NUCL]Physics [physics]/Nuclear Theory [nucl-th]
[PHYS.NEXP] Physics [physics]/Nuclear Experiment [nucl-ex]
Astrophysics::High Energy Astrophysical Phenomena
Nuclear engineering
uranium mining
chemistry.chemical_element
Radiation
[PHYS.NEXP]Physics [physics]/Nuclear Experiment [nucl-ex]
01 natural sciences
germanium detector
Index Terms-Nuclear measurements
0103 physical sciences
Calibration
Gamma spectroscopy
[PHYS.PHYS.PHYS-INS-DET]Physics [physics]/Physics [physics]/Instrumentation and Detectors [physics.ins-det]
Electrical and Electronic Engineering
010306 general physics
Spectroscopy
010308 nuclear & particles physics
Detector
Gamma ray
Nuclear data
Uranium
Nuclear Energy and Engineering
chemistry
gamma-ray spectroscopy
MCNP6
Zdroj: ANIMMA 2017
ANIMMA 2017, Jun 2017, Liege, Belgium
IEEE Transactions on Nuclear Science
IEEE Transactions on Nuclear Science, 2018, 65 (9), pp.2533-2538. ⟨10.1109/TNS.2018.2797312⟩
ISSN: 0018-9499
Popis: International audience; AREVA Mines and the Nuclear Measurement Laboratory of CEA Cadarache are collaborating to improve the sensitivity and precision of uranium concentration evaluation by means of gamma-ray measurements. This paper reports gamma-ray spectra, recorded with two high-purity germanium detectors, on standard cement blocks with increasing uranium content, and the corresponding MCNP simulations. The detailed MCNP model of detectors and experimental setup has been validated by calculation vs. experiment comparisons. An optimization of detector MCNP models is presented in this paper, as well as a comparison of different nuclear data libraries to explain missing or exceeding peaks in the simulation. Energy shifts observed between the fluorescence X-rays produced by MCNP and atomic data are also investigated, as well as gamma backscattering and beta radiation effects. The validated numerical models will be used in further studies to develop new gamma-ray spectroscopy approaches aiming at reducing acquisition times, especially for ore samples with low uranium content.
Databáze: OpenAIRE