2022 roadmap on low temperature electrochemical CO2 reduction
| Autor: | Stephens, I.E.L., Chan, K., Bagger, A., Boettcher, S., Bonin, J., Boutin, E., Buckley, A.K., Buonsanti, R., Cave, E.R., Chang, X., Chee, S.W., Marques da Silva, A.H., Luna, P. de, Einsle, O., Endrodi, B., Escudero-Escribano, M., Ferreira, A.J.V. de, Figueiredo, M.C., Hahn, C., Hansen, K.U., Huassener, S., Hunegnaw, S., Huo, Z., Hwang, Y.J., Janaky, C., Jayathilake, B.S., Jiao, F., Jovanov, Z.P., Karimi, P., Koper, M.T.M., Kuhl, K.P., Woong, H., Liang, Z., Liu, X., Ma, S., Ma, M., Oh, H.S., Robert, M., Cuenva, B.R., Rossmeisl, J., Roy, C., Ryan, M.P., Sargent, E.H., Sebastián-Pascual, P., Seger, B., Steier, L., Strasser, P., Varela, A.S., Vos, R.E., Wang, X., Xu, B., Yadegari, H., Zhou, X. |
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| Přispěvatelé: | Inorganic Materials & Catalysis, EIRES Chem. for Sustainable Energy Systems |
| Jazyk: | angličtina |
| Rok vydání: | 2022 |
| Předmět: |
STRUCTURAL BASIS
mechanistic insights SELECTIVE ELECTROREDUCTION BIPOLAR MEMBRANES liquid fuel solar fuels Materials Science (miscellaneous) technoeconomic analysis ACCELERATED DISCOVERY carbon-dioxide capture Solar fuels electrocatalytic conversion METAL-ELECTRODES Materials Chemistry Electrochemistry electrocatalysis selective electroreduction accelerated discovery MECHANISTIC INSIGHTS SDG 7 - Affordable and Clean Energy metal-electrodes TECHNOECONOMIC ANALYSIS CARBON-DIOXIDE CAPTURE structural basis bipolar membranes General Energy 540 Chemie und zugeordnete Wissenschaften electrochemistry CO2 reduction ELECTROCATALYTIC CONVERSION Electrocatalysis LIQUID FUEL SDG 7 – Betaalbare en schone energie |
| Zdroj: | Stephens, I E L, Chan, K, Bagger, A, Boettcher, S W, Bonin, J, Boutin, E, Buckley, A K, Buonsanti, R, Cave, E R, Chang, X, Chee, S W, da Silva, A H M, de Luna, P, Einsle, O, Endrődi, B, Escudero-Escribano, M, Ferreira de Araujo, J V, Figueiredo, M C, Hahn, C, Hansen, K U, Haussener, S, Hunegnaw, S, Huo, Z, Hwang, Y J, Janáky, C, Jayathilake, B S, Jiao, F, Jovanov, Z P, Karimi, P, Koper, M T M, Kuhl, K P, Lee, W H, Liang, Z, Liu, X, Ma, S, Ma, M, Oh, H S, Robert, M, Cuenya, B R, Rossmeisl, J, Roy, C, Ryan, M P, Sargent, E H, Sebastián-Pascual, P, Seger, B, Steier, L, Strasser, P, Varela, A S, Vos, R E, Wang, X, Xu, B, Yadegari, H & Zhou, Y 2022, ' 2022 roadmap on low temperature electrochemical CO 2 reduction ', JPhys Energy, vol. 4, no. 4, 042003 . https://doi.org/10.1088/2515-7655/ac7823 Stephens, I E L, Chan, K, Bagger, A, Boettcher, S W, Bonin, J, Boutin, E, Buckley, A K, Buonsanti, R, Cave, E R, Chang, X, Chee, S W, da Silva, A H M, de Luna, P, Einsle, O, Endrodi, B, Escudero-Escribano, M, de Araujo, J V F, Figueiredo, M C, Hahn, C, Hansen, K U, Haussener, S, Hunegnaw, S, Huo, Z, Hwang, Y J, Janaky, C, Jayathilake, B S, Jiao, F, Jovanov, Z P, Karimi, P, Koper, M T M, Kuhl, K P, Lee, W H, Liang, Z, Liu, X, Ma, S, Ma, M, Oh, H-S, Robert, M, Cuenya, B R, Rossmeisl, J, Roy, C, Ryan, M P, Sargent, E H, Sebastian-Pascual, P, Seger, B, Steier, L, Strasser, P, Varela, A S, Vos, R E, Wang, X, Xu, B, Yadegari, H & Zhou, Y 2022, ' 2022 roadmap on low temperature electrochemical CO 2 reduction ', JPhys Energy, vol. 4, no. 4, 042003 . https://doi.org/10.1088/2515-7655/ac7823 JPhys Energy, 4(4):042003. IOP Publishing Ltd. JPhys Energy, 4(4):042003. IOP Publishing Ltd |
| ISSN: | 2515-7655 |
| Popis: | Electrochemical CO2 reduction (CO2R) is an attractive option for storing renewable electricity and for the sustainable production of valuable chemicals and fuels. In this roadmap, we review recent progress in fundamental understanding, catalyst development, and in engineering and scale-up. We discuss the outstanding challenges towards commercialization of electrochemical CO2R technology: energy efficiencies, selectivities, low current densities, and stability. We highlight the opportunities in establishing rigorous standards for benchmarking performance, advances in in operando characterization, the discovery of new materials towards high value products, the investigation of phenomena across multiple-length scales and the application of data science towards doing so. We hope that this collective perspective sparks new research activities that ultimately bring us a step closer towards establishing a low- or zero-emission carbon cycle. |
| Databáze: | OpenAIRE |
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