Relevance of Kondo physics for the temperature dependence of the bulk modulus in plutonium
Autor: | Jason C. Lashley, J. D. Thompson, J. M. Lawrence, Marc Janoschek, Mark D Lumsden, Eve Bauer, G. H. Lander, Douglas L. Abernathy |
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Jazyk: | angličtina |
Rok vydání: | 2017 |
Předmět: |
Physics
Bulk modulus Multidisciplinary Valence (chemistry) Condensed matter physics Magnetism chemistry.chemical_element 02 engineering and technology 021001 nanoscience & nanotechnology 01 natural sciences Plutonium chemistry 0103 physical sciences Neutron Letters 010306 general physics 0210 nano-technology Ground state Local moment |
Popis: | The recent PNAS paper by Migliori et al. (1) attempts to explain the unusually strong temperature dependence of the bulk modulus of fcc plutonium (δ-Pu) by use of the disordered local moment (DLM) model. It is our opinion that this approach does not correctly incorporate the dynamic magnetism of δ-Pu. First, we note that, contrary to the comments in Migliori et al. (1), the results of our recent inelastic neutron experiments (2) do not contradict the results of earlier experiments (3⇓–5), which show that the ground state is nonmagnetic. All of these experiments are consistent with the interpretation that δ-Pu has a nonmagnetic fluctuating valence ground state. … [↵][1]1To whom correspondence should be addressed. Email: mjanoschek{at}lanl.gov. [1]: #xref-corresp-1-1 |
Databáze: | OpenAIRE |
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