Relevance of Kondo physics for the temperature dependence of the bulk modulus in plutonium

Autor: Jason C. Lashley, J. D. Thompson, J. M. Lawrence, Marc Janoschek, Mark D Lumsden, Eve Bauer, G. H. Lander, Douglas L. Abernathy
Jazyk: angličtina
Rok vydání: 2017
Předmět:
Popis: The recent PNAS paper by Migliori et al. (1) attempts to explain the unusually strong temperature dependence of the bulk modulus of fcc plutonium (δ-Pu) by use of the disordered local moment (DLM) model. It is our opinion that this approach does not correctly incorporate the dynamic magnetism of δ-Pu. First, we note that, contrary to the comments in Migliori et al. (1), the results of our recent inelastic neutron experiments (2) do not contradict the results of earlier experiments (3⇓–5), which show that the ground state is nonmagnetic. All of these experiments are consistent with the interpretation that δ-Pu has a nonmagnetic fluctuating valence ground state. … [↵][1]1To whom correspondence should be addressed. Email: mjanoschek{at}lanl.gov. [1]: #xref-corresp-1-1
Databáze: OpenAIRE