Novel insights on new particle formation derived from a pan-european observing system
| Autor: | Karine Sellegri, F. Bianchi, Monica Crippa, André S. H. Prévôt, Claire Granier, Annele Virtanen, Axel Eriksson, Roy M. Harrison, G. de Leeuw, James Allan, J. P. Putaud, J. S. Henzing, Liqing Hao, Erik Swietlicki, Rafel Simó, Manuel Dall'Osto, Hans-Christen Hansson, Paolo Laj, Colin D. O'Dowd, Laurent Poulain, Maria Vidal, Timothy B. Onasch, Manjula R. Canagaratna, David C. S. Beddows, Ari Asmi, Douglas R. Worsnop, Markku Kulmala, K. Zemankova, Evelyn Freney |
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| Přispěvatelé: | Spanish National Research Council (CSIC), National Centre for Atmospheric Science, University of Birmingham [Birmingham], Finnish Meteorological Institute (FMI), Leibniz Institute for Tropospheric Research (TROPOS), University of Eastern Finland, Laboratoire de météorologie physique (LaMP), Centre National de la Recherche Scientifique (CNRS)-Université Blaise Pascal - Clermont-Ferrand 2 (UBP)-Institut national des sciences de l'Univers (INSU - CNRS), European Commission - Joint Research Centre [Petten], University of Helsinki, Lund University [Lund], Laboratoire d'aérologie (LAERO), Centre National de la Recherche Scientifique (CNRS)-Observatoire Midi-Pyrénées (OMP), Météo France-Centre National d'Études Spatiales [Toulouse] (CNES)-Université Fédérale Toulouse Midi-Pyrénées-Centre National de la Recherche Scientifique (CNRS)-Institut de Recherche pour le Développement (IRD)-Météo France-Centre National d'Études Spatiales [Toulouse] (CNES)-Université Fédérale Toulouse Midi-Pyrénées-Centre National de la Recherche Scientifique (CNRS)-Institut de Recherche pour le Développement (IRD)-Université Toulouse III - Paul Sabatier (UT3), Université Fédérale Toulouse Midi-Pyrénées, Department of Applied Mathematics and Institute of Theoretical Computer Science (Charles University), Charles University [Prague] (CU), Institut des Géosciences de l’Environnement (IGE), Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP )-Institut de Recherche pour le Développement (IRD)-Université Grenoble Alpes [2016-2019] (UGA [2016-2019]), Aerodyne Research Inc., European Project: 36071,EUCAARI, European Project: 624680,EC:FP7:PEOPLE,FP7-PEOPLE-2013-IOF,MANU(2014), Department of Physics, Polar and arctic atmospheric research (PANDA), Centre National de la Recherche Scientifique (CNRS)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Blaise Pascal - Clermont-Ferrand 2 (UBP), Laboratoire d'aérologie (LA), Université Fédérale Toulouse Midi-Pyrénées-Université Fédérale Toulouse Midi-Pyrénées-Université Toulouse III - Paul Sabatier (UT3), Charles University [Prague], Laboratoire de glaciologie et géophysique de l'environnement (LGGE), Observatoire des Sciences de l'Univers de Grenoble (OSUG), Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP)-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Université Joseph Fourier - Grenoble 1 (UJF)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes (UGA)-Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry])-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP)-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Université Joseph Fourier - Grenoble 1 (UJF)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes (UGA)-Centre National de la Recherche Scientifique (CNRS), Université Blaise Pascal - Clermont-Ferrand 2 (UBP)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS), Helsingin yliopisto = Helsingfors universitet = University of Helsinki, Université Toulouse III - Paul Sabatier (UT3), Université de Toulouse (UT)-Université de Toulouse (UT)-Observatoire Midi-Pyrénées (OMP), Institut de Recherche pour le Développement (IRD)-Université Toulouse III - Paul Sabatier (UT3), Université de Toulouse (UT)-Université de Toulouse (UT)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Institut de Recherche pour le Développement (IRD)-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National d'Études Spatiales [Toulouse] (CNES)-Centre National de la Recherche Scientifique (CNRS)-Météo-France -Centre National de la Recherche Scientifique (CNRS), Institut de Recherche pour le Développement (IRD)-Institut polytechnique de Grenoble - Grenoble Institute of Technology (Grenoble INP )-Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université Grenoble Alpes [2016-2019] (UGA [2016-2019]), Universitat de Barcelona, Federal Office for the Environment (Switzerland), Ministerio de Economía y Competitividad (España), European Commission, Natural Environment Research Council (UK) |
| Jazyk: | angličtina |
| Rok vydání: | 2018 |
| Předmět: |
Statistical cluster
010504 meteorology & atmospheric sciences BIOGENIC EMISSIONS Growth phase Earth science Seasonal variation education AIR-QUALITY lcsh:Medicine Urbanisation 010501 environmental sciences Environment VOLATILE ORGANIC-COMPOUNDS CHEMICAL-COMPOSITION 01 natural sciences 7. Clean energy 114 Physical sciences Article CLOUD CONDENSATION NUCLEI Cluster analysis Pan european Growth curve SULFURIC-ACID ATMOSPHERIC NUCLEATION Contaminació atmosfèrica Ozó atmosfèric Cloud condensation nuclei lcsh:Science Aerosol POSITIVE MATRIX FACTORIZATION ComputingMilieux_MISCELLANEOUS 0105 earth and related environmental sciences [SDU.OCEAN]Sciences of the Universe [physics]/Ocean Atmosphere Multidisciplinary Atmospheric pollution SIZE DISTRIBUTIONS Biogenic emissions lcsh:R AEROSOL MASS-SPECTROMETER Atmospheric ozone Europe 13. Climate action [SDU]Sciences of the Universe [physics] Atmospheric chemistry Particle Environmental science lcsh:Q Environment & Sustainability |
| Zdroj: | Scientific Reports Scientific Reports, Nature Publishing Group, 2018, 8 (1), ⟨10.1038/s41598-017-17343-9⟩ Scientific Reports, 2018, 8 (1), ⟨10.1038/s41598-017-17343-9⟩ Recercat. Dipósit de la Recerca de Catalunya instname Dall'Osto, M, Beddows, D C S, Asmi, A, Poulain, L, Hao, L, Freney, E, Allan, J D, Canagaratna, M, Crippa, M, Bianchi, F, De Leeuw, G, Eriksson, A, Swietlicki, E, Hansson, H C, Henzing, J S, Granier, C, Zemankova, K, Laj, P, Onasch, T, Prevot, A, Putaud, J P, Sellegri, K, Vidal, M, Virtanen, A, Simo, R, Worsnop, D, O'Dowd, C, Kulmala, M & Harrison, R M 2018, ' Novel insights on new particle formation derived from a pan-european observing system ', Scientific Reports, vol. 8, no. 1, 1482 . https://doi.org/10.1038/s41598-017-17343-9 Scientific Reports, 1, 8 Digital.CSIC. Repositorio Institucional del CSIC Scientific Reports, Vol 8, Iss 1, Pp 1-11 (2018) Dipòsit Digital de la UB Universidad de Barcelona |
| ISSN: | 2045-2322 |
| DOI: | 10.1038/s41598-017-17343-9⟩ |
| Popis: | Dall'Osto, Manuel ... et al.-- 11 pages, 4 figures, supplementary material https://dx.doi.org/10.1038/s41598-017-17343-9 The formation of new atmospheric particles involves an initial step forming stable clusters less than a nanometre in size (~10 nm). Although at times, the same species can be responsible for both processes, it is thought that more generally each step comprises differing chemical contributors. Here, we present a novel analysis of measurements from a unique multi-station ground-based observing system which reveals new insights into continental-scale patterns associated with new particle formation. Statistical cluster analysis of this unique 2-year multi-station dataset comprising size distribution and chemical composition reveals that across Europe, there are different major seasonal trends depending on geographical location, concomitant with diversity in nucleating species while it seems that the growth phase is dominated by organic aerosol formation. The diversity and seasonality of these events requires an advanced observing system to elucidate the key processes and species driving particle formation, along with detecting continental scale changes in aerosol formation into the future We gratefully acknowledge support by the German Federal Environment Agency (Umweltbundesamt), grants no. 351 03 031 and 351 01 038, and UFOPLAN grant 3703 43 200 (title “Erfassung der Zahl feiner und ultrafeiner Partikel in der Außenluft”). [...] The study was funded by the Spanish Ministry of Economy through projects BIO-NUC (CGL2013-49020-R), and by the EU though the FP7-PEOPLE-2013-IOF programme (Project number 624680, MANU – Marine Aerosol NUcleations) and the Ramon y Cajal fellowship (RYC-2012-11922).The National Centre for Atmospheric Science NCAS Birmingham group is funded by the UK Natural Environment Research Council |
| Databáze: | OpenAIRE |
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