Unveiling hidden ferrimagnetism and giant magnetoelectricity in polar magnet Fe2Mo3O8

Autor: Yazhong Wang, Valery Kiryukhin, Kristjan Haule, G. L. Pascut, Sang-Wook Cheong, Bin Gao, Trevor A. Tyson
Rok vydání: 2015
Předmět:
Zdroj: Scientific Reports
ISSN: 2045-2322
Popis: Magnetoelectric (ME) effect is recognized for its utility for low-power electronic devices. Largest ME coefficients are often associated with phase transitions in which ferroelectricity is induced by magnetic order. Unfortunately, in these systems, large ME response is revealed only upon elaborate poling procedures. These procedures may become unnecessary in single-polar-domain crystals of polar magnets. Here we report giant ME effects in a polar magnet Fe2Mo3O8 at temperatures as high as 60 K. Polarization jumps of 0.3 μC/cm2 and repeated mutual control of ferroelectric and magnetic moments with differential ME coefficients on the order of 104 ps/m are achieved. Importantly, no electric or magnetic poling is needed, as necessary for applications. The sign of the ME coefficients can be switched by changing the applied “bias” magnetic field. The observed effects are associated with a hidden ferrimagnetic order unveiled by application of a magnetic field.
Databáze: OpenAIRE