Multiphoton-absorption induced ultraviolet luminescence of ZnO nanorods using low energy femtosecond pulses

Autor: Martin Bock, Enda McGlynn, Ruediger Grunwald, Markus Breusing, Mahua Biswas, Susanta Kumar Das, Daragh Byrne
Jazyk: angličtina
Rok vydání: 2010
Předmět:
Zdroj: Kumar Das, Susanta, Biswas, Mahua, Byrne, Daragh ORCID: 0000-0002-2040-9765 , Bock, Martin, McGlynn, Enda ORCID: 0000-0002-3412-9035 , Breusing, Markus and Grunwald, Rüdiger ORCID: 0000-0003-4822-2932 (2010) Multiphoton-absorption induced ultraviolet luminescence of ZnO nanorods using low energy femtosecond pulses. Journal of Applied Physics, 108 . 043107-043107. ISSN 0021-8979
Popis: Multiphoton-absorption (MPA) induced ultraviolet (UV) luminescence of ZnO nanorods grown by vapor phase transport was demonstrated using ultrafast excitation at pulse energies in the few nanojoules range, directly generated by a Ti:sapphire laser oscillator at wavelengths around 800 nm. The dependence of the UV luminescence on the excitation density reveals a two-photon absorption process as the responsible excitation mechanism. The broad spectral bandwidth of the excitation pulses obviously promotes the feasibility of the observed two-photon channel. Theoretical estimates concerning the contribution of nonlinear absorbance strongly support the experimental findings. The essential conditions for proper utilization of this process are discussed.
Databáze: OpenAIRE