Multicatalytic Hybrid Materials for Biocatalytic and Chemoenzymatic Cascades—Strategies for Multicatalyst (Enzyme) Co-Immobilization

Autor: Rodrigo O. M. A. de Souza, Ivaldo Itabaiana, Yan Ferraz Ximenes Ladeira, Aldo Araújo da Trindade Júnior, Alexandre da Silva França, Adolfo Henrique Moraes, Robert Wojcieszak, Amanda S. de Miranda
Přispěvatelé: Universidade Federal do Rio de Janeiro (UFRJ), Unité de Catalyse et Chimie du Solide - UMR 8181 (UCCS), Centrale Lille Institut (CLIL)-Université d'Artois (UA)-Centrale Lille-Centre National de la Recherche Scientifique (CNRS)-Institut de Chimie du CNRS (INC)-Université de Lille, CNRS, Centrale Lille, ENSCL, Univ. Artois, Université de Lille, Universidade Federal do Estado do Rio de Janeiro [UNIRIO], Universidade Federal de Minas Gerais [UFMG], Unité de Catalyse et Chimie du Solide (UCCS) - UMR 8181, Université d'Artois (UA)-Centrale Lille-Institut de Chimie du CNRS (INC)-Université de Lille-Centre National de la Recherche Scientifique (CNRS), ANR-16-IDEX-0004,ULNE,ULNE(2016)
Jazyk: angličtina
Rok vydání: 2021
Předmět:
Zdroj: Catalysts, Vol 11, Iss 936, p 936 (2021)
Catalysts
Catalysts, MDPI, 2021, 11 (8), ⟨10.3390/catal11080936⟩
Catalysts, 2021, 11 (8), ⟨10.3390/catal11080936⟩
ISSN: 2073-4344
DOI: 10.3390/catal11080936⟩
Popis: International audience; During recent decades, the use of enzymes or chemoenzymatic cascades for organic chemistry has gained much importance in fundamental and industrial research. Moreover, several enzymatic and chemoenzymatic reactions have also served in green and sustainable manufacturing processes especially in fine chemicals, pharmaceutical, and flavor/fragrance industries. Unfortu- nately, only a few processes have been applied at industrial scale because of the low stabilities of enzymes along with the problematic processes of their recovery and reuse. Immobilization and co-immobilization offer an ideal solution to these problems. This review gives an overview of all the pathways for enzyme immobilization and their use in integrated enzymatic and chemoenzymatic processes in cascade or in a one-pot concomitant execution. We place emphasis on the factors that must be considered to understand the process of immobilization. A better understanding of this fundamental process is an essential tool not only in the choice of the best route of immobilization but also in the understanding of their catalytic activity.
Databáze: OpenAIRE