Fluctuation-induced interactions and the spin-glass transition inFe2TiO5

Autor: Theo Siegrist, Sergey Syzranov, Arthur P. Ramirez, D. Phelan, Tiglet Besara, Yan Xin, P. G. LaBarre, S. Rosenkranz, Feng Ye
Rok vydání: 2021
Předmět:
Zdroj: Physical Review B. 103
ISSN: 2469-9969
2469-9950
Popis: We investigate the spin-glass transition in the strongly frustrated well-known compound $Fe_2TiO_5$. A remarkable feature of this transition, widely discussed in the literature, is its anisotropic properties: the transition manifests itself in the magnetic susceptibly only along one axis, despite $Fe^{3+}$ $d^5$ spins having no orbital component. We demonstrate, using neutron scattering, that below the transition temperature $T_g = 55 K$, $Fe_2TiO_5$ develops nanoscale surfboard shaped antiferromagnetic regions in which the $Fe^{3+}$ spins are aligned perpendicular to the axis which exhibits freezing. We show that the glass transition may result from the freezing of transverse fluctuations of the magnetization of these regions and we develop a mean-field replica theory of such a transition, revealing a type of magnetic van der Waals effect.
14 pages, 4 figures, 6 page supplemental material, 2 figures
Databáze: OpenAIRE