Technologies comparison for iterative data acquisition strategies
| Autor: | Commenge Jean-Marc, Mathieu Florent, Lomel Sébastien, Falk Laurent |
|---|---|
| Přispěvatelé: | Laboratoire Réactions et Génie des Procédés (LRGP), Université de Lorraine (UL)-Centre National de la Recherche Scientifique (CNRS), Centre National de la Recherche Scientifique (CNRS)-Université de Lorraine (UL) |
| Rok vydání: | 2013 |
| Předmět: |
Work (thermodynamics)
Computer science Estimation theory Applied Mathematics General Chemical Engineering Reaction scheme Experimental data Window (computing) ComputerApplications_COMPUTERSINOTHERSYSTEMS Control engineering 02 engineering and technology General Chemistry 010402 general chemistry 01 natural sciences Industrial and Manufacturing Engineering 0104 chemical sciences Experimental strategy Data acquisition 020401 chemical engineering [CHIM]Chemical Sciences Physics::Chemical Physics 0204 chemical engineering Plug flow reactor model |
| Zdroj: | Chemical Engineering Science Chemical Engineering Science, Elsevier, 2013, 104, pp.829-838. ⟨10.1016/j.ces.2013.09.053⟩ |
| ISSN: | 0009-2509 |
| DOI: | 10.1016/j.ces.2013.09.053 |
| Popis: | International audience; The present work proposes a new experimental strategy based on a general model which describes and includes different reactor technologies. The strategy is based on a sequential iterative approach where, in a predictive step, the model is used to propose optimal experimental conditions, and, in a validation step, experimental data are used to improve the parameter estimation. A specific work bench with three types of reactors (batch, semi-batch stirred tank and continuous plug flow reactor) has been developed. The demonstration of the strategy is performed by using a classical parallel-consecutive reaction scheme, for which it has been demonstrated experimentally that the use of several reactors enlarges the experimental window, which enables to improve the accuracy on kinetic constants by comparison to using a restricted experimental window, with only one kind of reactor. |
| Databáze: | OpenAIRE |
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