Effects of film growth kinetics on grain coarsening and grain shape
| Autor: | F. D. A. Aarão Reis |
|---|---|
| Rok vydání: | 2017 |
| Předmět: |
Surface diffusion
Materials science Condensed matter physics Nucleation 02 engineering and technology 021001 nanoscience & nanotechnology 01 natural sciences Power law Grain size Grain growth 0103 physical sciences Radius of gyration Grain boundary 010306 general physics 0210 nano-technology Grain boundary strengthening |
| Zdroj: | Physical review. E. 95(4-1) |
| ISSN: | 2470-0053 1539-3755 |
| Popis: | We study models of grain nucleation and coarsening during the deposition of a thin film using numerical simulations and scaling approaches. The incorporation of new particles in the film is determined by lattice growth models in three different universality classes, with no effect of the grain structure. The first model of grain coarsening is similar to that proposed by Saito and Omura [Phys. Rev. E 84, 021601 (2011)PLEEE81539-375510.1103/PhysRevE.84.021601], in which nucleation occurs only at the substrate, and the grain boundary evolution at the film surface is determined by a probabilistic competition of neighboring grains. The surface grain density has a power-law decay, with an exponent related to the dynamical exponent of the underlying growth kinetics, and the average radius of gyration scales with the film thickness with the same exponent. This model is extended by allowing nucleation of new grains during the deposition, with constant but small rates. The surface grain density crosses over from the initial power law decay to a saturation; at the crossover, the time, grain mass, and surface grain density are estimated as a function of the nucleation rate. The distributions of grain mass, height, and radius of gyration show remarkable power law decays, similar to other systems with coarsening and particle injection, with exponents also related to the dynamical exponent. The scaling of the radius of gyration with the height h relative to the base of the grain show clearly different exponents in growth dominated by surface tension and growth dominated by surface diffusion; thus it may be interesting for investigating the effects of kinetic roughening on grain morphology. In growth dominated by surface diffusion, the increase of grain size with temperature is observed. |
| Databáze: | OpenAIRE |
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