Multielectron effects in strong-field ionization of the oriented OCS molecule

Autor:	Mahmoud Abu-samha, Lars Bojer Madsen
Rok vydání:	2020
Předmět:	Physics Strong field Polarization (waves) 01 natural sciences 010305 fluids & plasmas Laser polarization Dipole Polarizability Ionization 0103 physical sciences Physics::Atomic and Molecular Clusters Molecule Molecular orbital Physics::Chemical Physics Atomic physics 010306 general physics
Zdroj:	Abu-Samha, M & Madsen, L B 2020, ' Multielectron effects in strong-field ionization of the oriented OCS molecule ', Physical Review A, vol. 102, no. 6, 063111 . https://doi.org/10.1103/PhysRevA.102.063111
ISSN:	2469-9934 2469-9926
DOI:	10.1103/physreva.102.063111
Popis:	We present theoretical calculations of orientation-dependent total ionization yields from the highest occupied molecular orbitals of the oriented OCS molecule by solving the time-dependent Schr\"odinger equation in three dimensions. The calculations were performed within the single-active-electron approximation including multielectron polarization. The multielectron polarization term was represented by an induced dipole term which contains the polarizability of the ${\mathrm{OCS}}^{+}$ cation parallel to the laser polarization. Upon accounting for multielectron polarization, the calculated total ionization yields and their orientation dependence are in good agreement with experimental data.
Databáze:	OpenAIRE
Externí odkaz:	https://explore.openaire.eu/search/publication?articleId=doi_dedup___::a90f7fa0c76deca2aa8f6f0a3ba82b1d https://doi.org/10.1103/physreva.102.063111 Zobrazit plný text záznamu