Characteristics and Source Analysis of Trace Elements in PM2.5 in the Urban Atmosphere of Wuhan in Spring
Autor: | Costanza Acciai, Zhenyi Zhang, Zhangxiong Zhong, Giovanni Lonati, Fenjuan Wang |
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Rok vydání: | 2017 |
Předmět: |
geography
geography.geographical_feature_category 010504 meteorology & atmospheric sciences Period (periodic table) Trace element Central china Storm 010501 environmental sciences 01 natural sciences Pollution Ambient air Atmosphere Environmental chemistry Spring (hydrology) Environmental Chemistry Environmental science Enrichment factor 0105 earth and related environmental sciences |
Zdroj: | Aerosol and Air Quality Research. 17:2224-2234 |
ISSN: | 2071-1409 1680-8584 |
Popis: | The concentrations of PM2.5 and trace elements with hourly resolution were measured during May 2014 in urban residential area of Wuhan, the biggest city in central China. During the period of measurement, the average temperature was approximate 25°C without domestic heating and cooling. The average concentration of PM2.5 was 95.53 μg m^(-3), which was higher than the limit of Ambient Air Quality Standard of China GB3095-2012 (75 μg m^(-3), Level 2). A sand storm original from Northwestern China was also recorded. Concentrations of major trace elements (K, Ca, V, Cr, Mn, Fe, Ni, Cu, Zn, Ga, As, Se, Pd, Ag, Cd, Au, Hg, Pb, Co, Sn, Sb, Tl) were comparable to previous studies, except for Ba and Ca with more than doubled concentrations (103 ng m^(-3), 1,792.49 ng m^(-3)) due to the storm. Enrichment Factor (EF) and Positive Matrix Factorization (PMF) were employed to characterize the emission sources. The computation of EF showed that Zincs was highly enriched. Four sources, biomass burning (63.2%) might mainly related to power plants using bio-waste burning and bio-related cooking activities, metallurgical and steel industries (14%), dust crustal (12.5%) and dust associated with vehicular traffic (10.4%), were identified in decreasing order of average percentage contribution to the PM2.5 mass with the aid of trace elements. The orientations of emission sources were also addressed. |
Databáze: | OpenAIRE |
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