Bismuth ferrite dielectric nanoparticles excited at telecom wavelengths as multicolor sources by second, third, and fourth harmonic generation

Autor: Luigi Bonacina, Cédric Schmidt, Tadas Balciunas, Andrius Baltuška, Yannick Mugnier, Alexis Demierre, Gabriel Campargue, Ronan Le Dantec, Jean-Pierre Wolf, Jérémy Riporto, Vasyl Kilin, Mathias Urbain
Přispěvatelé: Laboratoire SYstèmes et Matériaux pour la MEcatronique (SYMME), Université Savoie Mont Blanc (USMB [Université de Savoie] [Université de Chambéry]), Université de Genève (UNIGE)
Rok vydání: 2018
Předmět:
Zdroj: Nanoscale
Nanoscale, Royal Society of Chemistry, 2018, 10 (17), pp.8146-8152. ⟨10.1039/C7NR08102B⟩
Nanoscale, Vol. 10, No 17 (2018) pp. 8146-8152
ISSN: 2040-3372
2040-3364
Popis: We demonstrate the simultaneous generation of second, third, and fourth harmonic from a single dielectric Bismuth Ferrite nanoparticle excited by a telecom fiber laser at 1560 nm. We first characterize the signals associated with different nonlinear orders in terms of spectrum, excitation intensity dependence, and relative signal strengths. Successively, on the basis of the polarization-resolved emission curves of the three harmonics, we discuss the interplay of susceptibility tensor components at the different orders and we show how polarization can be used as an optical handle to control the relative frequency conversion properties.
Comment: include S.I. section at the end of the main pdf file
Databáze: OpenAIRE