Manipulating Interactions between Dielectric Particles with Electric Fields: A General Electrostatic Many-Body Framework

Autor: Muhammad Hassan, Connor Williamson, Joshua Baptiste, Stefanie Braun, Anthony J. Stace, Elena Besley, Benjamin Stamm
Jazyk: angličtina
Rok vydání: 2022
Předmět:
ISSN: 1549-9618
1549-9626
Popis: We derive a rigorous analytical formalism and propose a numerical method for the quantitative evaluation of the electrostatic interactions between dielectric particles in an external electric field. This formalism also allows for inhomogeneous charge distributions, and, in particular, for the presence of pointlike charges on the particle surface. The theory is based on a boundary integral equation framework and yields analytical expressions for the interaction energy and net forces that can be computed in linear scaling cost, with respect to the number of interacting particles. We include numerical results that validate the proposed method and show the limitations of the fixed dipole approximation at small separation between interacting particles. The proposed method is also applied to study the stability and melting of ionic colloidal crystals in an external electric field.
Databáze: OpenAIRE