Nondestructive Femtosecond Laser Lithography of Ni Nanocavities by Controlled Thermo-Mechanical Spallation at the Nanoscale

Autor: Vadim P. Veiko, Evgeny Modin, Dmitry S. Ivanov, Alexandr Alekhin, Alexey M. Lomonosov, Paolo Vavassori, Vasily V. Temnov, A. A. Samokhvalov
Přispěvatelé: Institut des Molécules et Matériaux du Mans (IMMM), Le Mans Université (UM)-Institut de Chimie du CNRS (INC)-Centre National de la Recherche Scientifique (CNRS), National Research University of Information Technologies, Mechanics and Optics [St. Petersburg] (ITMO), A. M. Prokhorov General Physics Institute (GPI), Russian Academy of Sciences [Moscow] (RAS), CICNanoGUNE
Jazyk: angličtina
Rok vydání: 2020
Předmět:
Materials science
genetic structures
Magnetism
Physics::Optics
FOS: Physical sciences
Bioengineering
02 engineering and technology
Applied Physics (physics.app-ph)
7. Clean energy
Fluence
law.invention
[SPI]Engineering Sciences [physics]
law
Mesoscale and Nanoscale Physics (cond-mat.mes-hall)
General Materials Science
Spallation
[NLIN]Nonlinear Sciences [physics]
Lithography
[PHYS]Physics [physics]
Condensed Matter - Materials Science
Laser ablation
Condensed Matter - Mesoscale and Nanoscale Physics
business.industry
Mechanical Engineering
Materials Science (cond-mat.mtrl-sci)
General Chemistry
Physics - Applied Physics
021001 nanoscience & nanotechnology
Condensed Matter Physics
Laser
eye diseases
Femtosecond
Optoelectronics
sense organs
0210 nano-technology
business
Maskless lithography
Optics (physics.optics)
Physics - Optics
Zdroj: Nano Letters
Nano Letters, American Chemical Society, 2020, ⟨10.1021/acs.nanolett.0c02574⟩
ISSN: 1530-6984
1530-6992
DOI: 10.1021/acs.nanolett.0c02574⟩
Popis: We present a new approach to femtosecond direct laser writing lithography to pattern nanocavities in ferromagnetic thin films. To demonstrate the concept we irradiated 300~nm thin nickel films by single intense femtosecond laser pulses through the glass substrate and created complex surface landscapes at the nickel-air interface. Using a fluence above the ablation threshold the process is destructive and irradiation leads to the formation of 200~nm thin flakes of nickel around the ablation crater as seen by electron microscopy. By progressively lowering the peak laser fluence, slightly below the ablation threshold the formation of closed spallation cavities is demonstrated by interferometric microscopy. Systematic studies by electron and optical interferometric microscopies enabled us to gain an understanding of the thermo-mechanical mechanism leading to spallation at the solid-molten interface, a conclusion supported by molecular dynamics simulations. We achieved a control of the spallation process that enabled the fabrication of closed spallation nanocavities and their periodic arrangements. Due to their topology closed magnetic nanocavities can support unique couplings of multiple excitations (magnetic, optical, acoustic, spintronic). Thereby, they offer a unique physics playground, before unavailable, for magnetism, magneto-photonic and magneto-acoustic applications.
4 figures
Databáze: OpenAIRE