High efficiency ultrafast water-window harmonic generation for single-shot soft X-ray spectroscopy

Autor: Pengfei Lan, Kotaro Nishimura, Katsumi Midorikawa, Renzhi Shao, Yuxi Fu, Eiji J. Takahashi, Akira Suda
Jazyk: angličtina
Rok vydání: 2020
Předmět:
Zdroj: Communications Physics, Vol 3, Iss 1, Pp 1-10 (2020)
ISSN: 2399-3650
Popis: Fully coherent, soft X-ray attosecond pulses are now available through high-order harmonic generation (HHG); however, the output energy is insufficient for various applications, such as attosecond-scale soft X-ray nonlinear experiments, the seeding of soft X-ray free-electron lasers, attosecond-pump-attosecond-probe spectroscopies, and single-shot imaging. In this paper, we combine a newly developed TW class mid-infrared femtosecond laser and a loose focusing geometry for HHG. A soft X-ray harmonic beam up to the water window region is demonstrated, which is more than 100 times intense compared to previous works. We achieve a high conversion efficiency, low beam divergence and a significantly reduced medium gas pressure. As the first application, we demonstrate near edge X-ray absorption fine structure experiments with clear fine absorption spectra near the K- and L-edges observed. The robust energy scaling method on HHG opens the door for demonstrating single-shot absorption spectrum and live-cell imaging with a femtosecond time resolution. While high harmonic x-ray sources are well established sources for ultrafast spectroscopy, the decrease in efficiency towards higher energies limits their application. Here, a loose-focused, TW mid-IR laser is used to generate high harmonic soft x-rays with pulse energies of a few nJ in the water window and easy energy scaling.
Databáze: OpenAIRE
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