Ultrafast nonlinear transparency driven at a telecom wavelength in an organic semiconductor system

Autor: Ruth Shinar, Joseph Shinar, Zhaoyu Liu, Jigang Wang, Liang Luo, Fadzai Fungura, Di Cheng, Joong Mok Park, Aaron Patz, Kai-Ming Ho
Jazyk: angličtina
Rok vydání: 2019
Předmět:
Zdroj: AIP Advances, Vol 9, Iss 2, Pp 025303-025303-5 (2019)
ISSN: 2158-3226
Popis: Ultrafast laser-induced transparency is demonstrated using femtosecond (fs) pump-probe experiments in the organic P3HT:PCBM (donor:acceptor) blend structure. For above band gap pumping, ultrafast transient signals strongly depend on the probe photon energy. Most intriguingly, for below band gap pumping at 0.95 eV, or 1.3 µm at a telecom wavelength, a huge transmission increase up to 30% only during the laser pulse ∼100 fs is observed as a pump-driven, quasi-instantaneous suppression of absorption for the high photon-energy energy probe beam. We attribute the observed laser-driven transparency to dynamic Franz-Keldysh effect, at least one order of magnitude stronger compared to the multiphoton nonlinearities. Our results may be used for development of low-cost, beyond 100 Gbit/s optical switching devices.
Databáze: OpenAIRE