Impact of nitrate-enhanced leachate recirculation on gaseous releases from a landfill bioreactor cell
| Autor: | A. Budka, Chrystelle Bureau, D. Presse, J. C. Benoist, M. Lemunier, P. Peu, Théodore Bouchez, G. Tallec |
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| Přispěvatelé: | Hydrosystèmes et Bioprocédés (UR HBAN), Centre national du machinisme agricole, du génie rural, des eaux et forêts (CEMAGREF), Gestion environnementale et traitement biologique des déchets (UR GERE), SUEZ ENVIRONNEMENT (FRANCE), SITA FRANCE NANTERRE FRA, Partenaires IRSTEA, Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA)-Institut national de recherche en sciences et technologies pour l'environnement et l'agriculture (IRSTEA) |
| Jazyk: | angličtina |
| Rok vydání: | 2009 |
| Předmět: |
Nitrous Oxide
Analytical chemistry 010501 environmental sciences 01 natural sciences Methane law.invention 03 medical and health sciences chemistry.chemical_compound Bioreactors Biogas law Flame ionization detector Leachate Waste Management and Disposal 0105 earth and related environmental sciences Flame Ionization 0303 health sciences Nitrates 030306 microbiology Chemistry Nitrous oxide Carbon Dioxide equipment and supplies Dilution Oxygen Electron capture detector 13. Climate action Environmental chemistry Carbon dioxide [SDE]Environmental Sciences Volatilization |
| Zdroj: | Waste Management Waste Management, Elsevier, 2009, 29 (7), pp.2078-2084. ⟨10.1016/j.wasman.2009.01.006⟩ |
| ISSN: | 0956-053X |
| DOI: | 10.1016/j.wasman.2009.01.006⟩ |
| Popis: | This study evaluates the impact of nitrate injection on a full scale landfill bioreactor through the monitoring of gaseous releases and particularly N{sub 2}O emissions. During several weeks, we monitored gas concentrations in the landfill gas collection system as well as surface gas releases with a series of seven static chambers. These devices were directly connected to a gas chromatograph coupled to a flame ionisation detector and an electron capture detector (GC-FID/ECD) placed directly on the field. Measurements were performed before, during and after recirculation of raw leachate and nitrate-enhanced leachate. Raw leachate recirculation did not have a significant effect on the biogas concentrations (CO{sub 2}, CH{sub 4} and N{sub 2}O) in the gas extraction network. However, nitrate-enhanced leachate recirculation induced a marked increase of the N{sub 2}O concentrations in the gas collected from the recirculation trench (100-fold increase from 0.2 ppm to 23 ppm). In the common gas collection system however, this N{sub 2}O increase was no more detectable because of dilution by gas coming from other cells or ambient air intrusion. Surface releases through the temporary cover were characterized by a large spatial and temporal variability. One automated chamber gave limited standard errors over each experimental period formore » N{sub 2}O releases: 8.1 {+-} 0.16 mg m{sup -2} d{sup -1} (n = 384), 4.2 {+-} 0.14 mg m{sup -2} d{sup -1} (n = 132) and 1.9 {+-} 0.10 mg m{sup -2} d{sup -1} (n = 49), during, after raw leachate and nitrate-enhanced leachate recirculation, respectively. No clear correlation between N{sub 2}O gaseous surface releases and recirculation events were evidenced. Estimated N{sub 2}O fluxes remained in the lower range of what is reported in the literature for landfill covers, even after nitrate injection.« less |
| Databáze: | OpenAIRE |
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