Stacked wire-mesh monoliths for VOCs combustion: Effect of the mesh-opening in the catalytic performance
| Autor: | Mario Montes, Oihane Sanz, Antonio Monzón, Haizea Larumbe, Aintzane Goya, Juan José Delgado, Ezequiel D. Banús |
|---|---|
| Rok vydání: | 2017 |
| Předmět: |
Materials science
chemistry.chemical_element INGENIERÍAS Y TECNOLOGÍAS 02 engineering and technology Manganese 010402 general chemistry Combustion Molecular sieve 01 natural sciences Catalysis WIRE-MESH MONOLITHS Metal chemistry.chemical_compound PT/OMS-2 VOCS ABATEMENT Chromatography General Chemistry MESH-OPENING 021001 nanoscience & nanotechnology Toluene 0104 chemical sciences Bifunctional catalyst Ingeniería Química chemistry Chemical engineering visual_art Otras Ingeniería Química visual_art.visual_art_medium Methanol 0210 nano-technology |
| Zdroj: | Catalysis Today. 296:76-83 |
| ISSN: | 0920-5861 |
| DOI: | 10.1016/j.cattod.2017.05.054 |
| Popis: | Structured reactors based on low cost metallic wire-mesh substrates of highly enhanced transport properties can be an interesting alternative to parallel channel monolithic reactors. In this work stacked wire-mesh monoliths were studied for volatile organic compounds elimination. Monoliths of different mesh-opening were homogeneously and adherently dip-coated with Pt/Manganese Octahedral Molecular Sieve (OMS-2) bifunctional catalyst. The catalytic activity was tested in toluene and methanol complete oxidation reactions. Catalytic activity increases using stacked wire-mesh monoliths instead of parallel channel monoliths and decreases when increasing the wire-mesh opening, showing the importance of the mass-transfer phenomena (contact between the gas phase and the solid catalyst). Fil: Sanz, Oihane. Universidad del País Vasco; España Fil: Banus, Ezequiel David. Universidad del País Vasco; España. Consejo Nacional de Investigaciones Científicas y Técnicas. Centro Científico Tecnológico Conicet - Santa Fe. Instituto de Investigaciones en Catálisis y Petroquímica ; Argentina Fil: Goya, Aintzane. Universidad del País Vasco; España Fil: Larumbe, Haizea. Universidad del País Vasco; España Fil: Delgado, Juan José. Universidad de Cádiz; España Fil: Monzón, Antonio. Universidad de Cádiz; España Fil: Montes, Mario. Universidad del País Vasco; España |
| Databáze: | OpenAIRE |
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