Highly efficient and stable inverted perovskite solar cell employing PEDOT:GO composite layer as a hole transport layer

Autor: Soo-Min Baek, Kyoung Jin Choi, Eui Dae Jung, Sung Soo Park, Hong Ji A, Myoung Hoon Song, Jae Choul Yu, Shinuk Cho, Sukbin Lee, Da Bin Kim
Jazyk: angličtina
Rok vydání: 2018
Předmět:
Zdroj: Scientific Reports, Vol 8, Iss 1, Pp 1-9 (2018)
Scientific Reports
ISSN: 2045-2322
Popis: The beneficial use of a hole transport layer (HTL) as a substitution for poly(3,4-ethlyenedioxythiophene): polystyrene sulfonate (PEDOT:PSS) is regarded as one of the most important approaches for improving the stability and efficiency of inverted perovskite solar cells. Here, we demonstrate highly efficient and stable inverted perovskite solar cells by applying a GO-doped PEDOT:PSS (PEDOT:GO) film as an HTL. The high performance of this solar cell stems from the excellent optical and electrical properties of the PEDOT:GO film, including a higher electrical conductivity, a higher work function related to the reduced contact barrier between the perovskite layer and the PEDOT:GO layer, enhanced crystallinity of the perovskite crystal, and suppressed leakage current. Moreover, the device with the PEDOT:GO layer showed excellent long-term stability in ambient air conditions. Thus, the enhancement in the efficiency and the excellent stability of inverted perovskite solar cells are promising for the eventual commercialization of perovskite optoelectronic devices.
Databáze: OpenAIRE
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