Research Works on Iodine and Ruthenium Behavior in Severe Accident Conditions

Autor: T. Albiol, Juliette Colombani, C. Mun, Céline Monsanglant-Louvet, Marie-Noelle Ohnet, Christophe Volkringer, Anne-Cécile Grégoire, Bruno Azambre, Olivia Leroy, Frédéric Cousin, Florent Louis, L. Bosland, Laurent Cantrel, Sidi Souvi, Sandrine Morin
Přispěvatelé: Institut de Radioprotection et de Sûreté Nucléaire (IRSN), Physicochimie des Processus de Combustion et de l’Atmosphère - UMR 8522 (PC2A), Université de Lille-Centre National de la Recherche Scientifique (CNRS), Laboratoire de Chimie et Physique - Approche Multi-échelle des Milieux Complexes (LCP-A2MC), Université de Lorraine (UL), Unité de Catalyse et Chimie du Solide - UMR 8181 (UCCS), Centrale Lille Institut (CLIL)-Université d'Artois (UA)-Centrale Lille-Centre National de la Recherche Scientifique (CNRS)-Institut de Chimie du CNRS (INC)-Université de Lille, Pôle Sûreté Nucléaire - Recherche en sûreté (IRSN/PSN-RES), Université d'Artois (UA)-Centrale Lille-Institut de Chimie du CNRS (INC)-Université de Lille-Centre National de la Recherche Scientifique (CNRS), Université de Lille-Centre National de la Recherche Scientifique (CNRS)-Ecole Nationale Supérieure de Chimie de Lille (ENSCL)-Ecole Centrale de Lille-Université d'Artois (UA)
Jazyk: angličtina
Rok vydání: 2018
Předmět:
020209 energy
Nuclear engineering
Scrubber
chemistry.chemical_element
02 engineering and technology
7. Clean energy
law.invention
law
Nuclear power plant
0202 electrical engineering
electronic engineering
information engineering

Nuclear safety
Public acceptance
Process engineering
Nuclear knowledge management
Nuclear education
Design-basis event
ComputingMilieux_MISCELLANEOUS
Radiation
business.industry
021001 nanoscience & nanotechnology
Ruthenium
[CHIM.THEO]Chemical Sciences/Theoretical and/or physical chemistry
Nuclear Energy and Engineering
chemistry
Containment
Accident management
Nuclear Knowledge Management
Security
[PHYS.PHYS.PHYS-CHEM-PH]Physics [physics]/Physics [physics]/Chemical Physics [physics.chem-ph]
0210 nano-technology
business
[CHIM.RADIO]Chemical Sciences/Radiochemistry
Public Acceptance
Zdroj: Journal of Nuclear Engineering and Radiation Science
Journal of Nuclear Engineering and Radiation Science, ASME, 2018, 4 (2), 020903 (13 p.). ⟨10.1115/1.4038223⟩
Journal of Nuclear Engineering and Radiation Science, 2018, 4 (2), 020903 (13 p.). ⟨10.1115/1.4038223⟩
Journal of Nuclear Engineering and Radiation Science, ASME, 2018, ASME Journal of Nuclear Engineering and Radiation Science, 4, ⟨10.1115/1.4038223⟩
ISSN: 2332-8983
Popis: This paper deals with near past, ongoing, and planned R&D works on fission products (FPs) behavior in reactor cooling system (RCS), containment building and in filtered containment venting systems (FCVS) for severe accident (SA) conditions. All the researches are collaborative works; the overall objective is to develop confident models to be implemented in simulation software. After being initiated in 2004, researches on iodine transport through the RCS are still ongoing and for containment, the last advances are linked to the source term (ST) evaluation and mitigation (STEM) OECD/NEA project. The objective is to improve the evaluation of ST for a SA on a nuclear power plant and to reduce uncertainties on specific phenomena dealing with the chemistry of two major FPs: iodine and ruthenium. For ruthenium attention has been paid to study the amount and nature (gas/aerosol partition) of ruthenium species along the RCS. A follow-up, called STEM2, has started to reduce some remaining issues and be closer to reactor conditions. For FCVS works, the efficiencies for trapping iodine covering scrubbers and dry filters are examined to get a clear view of their abilities in SA conditions. Another part is focused on specific porous materials able to trap volatile iodine. Influence of zeolite materials parameters (nature of the counter-ions, structure, Si/Al ratio…) are tested as well as new kind of porous materials constituted by Metal organic Frameworks will also be looked at.
Databáze: OpenAIRE