High-Performance Organic Photovoltaics Incorporating an Active Layer with a Few Nanometer-Thick Third-Component Layer on a Binary Blend Layer
Autor: | Hao Cheng Wang, Chien Yao Juan, Yu Che Lin, Pei Cheng, Anisha Mohapatra, Yang Yang, Bin Chang, Kung-Hwa Wei, Chung Hao Chen, Chih-Wei Chu, Hao Wen Cheng |
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Rok vydání: | 2021 |
Předmět: |
Materials science
Organic solar cell business.industry Mechanical Engineering Bilayer Photovoltaic system Energy conversion efficiency Bioengineering 02 engineering and technology General Chemistry 021001 nanoscience & nanotechnology Condensed Matter Physics Active layer Optoelectronics General Materials Science Nanometre 0210 nano-technology business Ternary operation Layer (electronics) |
Zdroj: | Nano Letters. 21:2207-2215 |
ISSN: | 1530-6992 1530-6984 |
Popis: | In this paper, a universal approach toward constructing a new bilayer device architecture, a few-nanometer-thick third-component layer on a bulk-heterojunction (BHJ) binary blend layer, has been demonstrated in two different state-of-the-art organic photovoltaic (OPV) systems. Through a careful selection of a third component, the power conversion efficiency (PCE) of the device based on PM6/Y6/layered PTQ10 layered third-component structure was 16.8%, being higher than those of corresponding devices incorporating the PM6/Y6/PTQ10 BHJ ternary blend (16.1%) and the PM6/Y6 BHJ binary blend (15.5%). Also, the device featuring PM7/Y1-4F/layered PTQ10 layered third-component structure gave a PCE of 15.2%, which is higher than the PCEs of the devices incorporating the PM7/Y1-4F/PTQ10 BHJ ternary blend and the PM7/Y1-4F BHJ binary blend (14.2 and 14.0%, respectively). These enhancements in PCE based on layered third-component structure can be attributed to improvements in the charge separation and charge collection abilities. This simple concept of the layered third-component structure appears to have great promise for achieving high-performance OPVs. |
Databáze: | OpenAIRE |
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