Optically controlled magnetic-field etching on the nano-scale

Autor: Maiku Yamaguchi, Fabrice Stehlin, Katsuyuki Nobusada, Daniel Bloch, Olivier Soppera, Satoshi Tojo, Toshiki Tsuboi, Takashi Yatsui
Přispěvatelé: The University of Tokyo (UTokyo), Institute for Molecular Sciences, National Institutes of Natural Sciences, Department of Physics, Chuo University, Chuo University (Chuo University), Institut de Science des Matériaux de Mulhouse (IS2M), Université de Haute-Alsace (UHA) Mulhouse - Colmar (Université de Haute-Alsace (UHA))-Centre National de la Recherche Scientifique (CNRS), Laboratoire de Physique des Lasers (LPL), Université Paris 13 (UP13)-Centre National de la Recherche Scientifique (CNRS)
Rok vydání: 2016
Předmět:
Zdroj: Light: Science and Applications
Light: Science and Applications, Nature Publishing Group, 2016, ⟨10.1038/lsa.2016.54⟩
Light, Science & Applications
ISSN: 2047-7538
2095-5545
Popis: Electric and magnetic fields play an important role in both chemical and physical reactions. However, since the coupling efficiency between magnetic fields and electrons is low in comparison with that between electric fields and electrons in the visible wavelength region, the magnetic field is negligible in photo-induced reactions. Here, we performed photo-etching of ZrO2 nano-stripe structures, and identified an etching-property polarisation dependence. Specifically, the etching rate and etched profiles depend on the structure width. To evaluate this polarisation-dependent etching, we performed numerical calculations using a finite-difference time-domain method. Remarkably, the numerical results revealed that the polarisation-dependent etching properties were determined by the magnetic field distributions, rather than the electric field distributions. As nano-scale structures induce a localised magnetic field, the discovery of this etching dependence on the magnetic field is expected to introduce a new perspective on advanced nano-scale structure fabrication. The magnetic-field polarization of incident light has been found to affect photoetching of zirconium oxide (ZrO2) nanostripes. Takashi Yatsui of the University of Tokyo and co-workers in Japan and France have found that the etching rates and the profiles of etched structures depended on the incident polarization. Numerical calculations revealed that this polarization dependence of the etching properties stemmed from the distribution of the magnetic field rather than that of the electric field. This is a surprising result since the magnetic field is generally ignored in light-induced reactions because it is considered to have negligible interaction with materials due to its low coupling efficiency with the electrons in a material. The inclusion of the magnetic field will provide an extra degree of freedom when fabricating nanostructures for advanced optical and electrical devices.
Databáze: OpenAIRE