Insights into the mechanism of carbon chain growth on zeolite-based Fischer–Tropsch Co/Y catalysts

Autor:	Xiuqin Dong, Jiaqi Li, Tianfeng Ma, Lingtao Wang
Rok vydání:	2022
Předmět:	General Physics and Astronomy Physical and Theoretical Chemistry
Zdroj:	Physical Chemistry Chemical Physics. 24:14751-14762
ISSN:	1463-9084 1463-9076
DOI:	10.1039/d2cp01287a
Popis:	In a zeolite-based Fischer-Tropsch bifunctional catalyst, zeolites, as the support of the active metal, can interact with the metal cluster to affect the electronic properties and structural effect of the catalyst, thus affecting the Fischer-Tropsch synthesis reaction. In this work, the Fischer-Tropsch synthesis process using a Co catalyst supported by Y-zeolite was simulated by the DFT method from the microscopic point of view. The reaction network was designed to investigate the reaction mechanism in terms of four parts consisting of H-assisted CO dissociation, C
Databáze:	OpenAIRE
Externí odkaz:	https://explore.openaire.eu/search/publication?articleId=doi_dedup___::3fcf6552058e9ba2c09adab7ca6b5979 https://doi.org/10.1039/d2cp01287a Zobrazit plný text záznamu