Water-soluble inorganic ions in urban aerosols of the continental part of Balkans (Belgrade) during the summer – autumn (2008)
Autor: | Dubravka Relić, Ljubiša M. Ignjatović, Maria A. Stortini, Ivana Tošić, Dragana Đorđević, Andrea Gambaro, Aleksandra Mihajlidi-Zelić |
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Jazyk: | angličtina |
Rok vydání: | 2014 |
Předmět: |
Mediterranean climate
Balkan region 010504 meteorology & atmospheric sciences Meteorology balkan region 010501 environmental sciences Inorganic ions Atmospheric sciences 01 natural sciences Materials Chemistry Mass concentration (chemistry) QD1-999 Air mass 0105 earth and related environmental sciences Urban aerosol urban aerosol Chemistry size-segregated inorganic ions General Chemistry Aerosol Size-segregated inorganic ions Water soluble Volume (thermodynamics) 13. Climate action HYSPLIT |
Zdroj: | Open Chemistry, Vol 13, Iss 1 (2014) Open Chemistry OPEN CHEMISTRY |
ISSN: | 2391-5420 |
Popis: | Size-segregated aerosol samples were collected using six stages High Volume Cascade Impactor. Aerosol mass and water soluble ions concentrations were determined. The Hybrid Single-Particle Lagrangian Integrated Trajectory (HYSPLIT) model was used to study the origin of air masses arriving to Belgrade in the investigated period. The obtained results of aerosol mass and water-soluble ion concentrations have been divided into six sub-data sets based on air mass categories. The highest average mass concentration of the fine mode (Dp ≤ 0.49 μm) was found for air masses coming to Belgrade from the southeast and northwest directions, and of the coarse mode (3.0 < Dp ≤7.2 μm) for air masses arriving from the northwest direction. The highest concentrations of SO4 2– were found in the fine particles transported to the investigated area by air masses from southeast direction. The analysis of contribution of marine aerosol components (Na+ and Cl-), the Correlation and Cluster Analysis indicated the influence of marine aerosol on urban aerosol of the central Balkans coming from the Western Mediterranean and northern direction. NH4 + and SO4 2- and K+ dominated in the fine mode for all air mass categories. PCA demonstrated the dominant impact of secondary aerosol formation processes on urban aerosols. |
Databáze: | OpenAIRE |
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