Advances in All-Inorganic Perovskite Nanocrystal-Based White Light Emitting Devices

Autor: Tajamul A. Wani, Javad Shamsi, Xinyu Bai, Neha Arora, M. Ibrahim Dar
Přispěvatelé: Shamsi, Javad [0000-0003-4684-5407], Dar, M Ibrahim [0000-0001-9489-8365], Apollo - University of Cambridge Repository
Rok vydání: 2023
Předmět:
Zdroj: ACS Omega. 8:17337-17349
ISSN: 2470-1343
DOI: 10.1021/acsomega.3c00188
Popis: Metal halide perovskites (MHPs) are exceptional semiconductors best known for their intriguing properties, such as high absorption coefficients, tunable bandgaps, excellent charge transport, and high luminescence yields. Among various MHPs, all-inorganic perovskites exhibit benefits over hybrid compositions. Notably, critical properties, including chemical and structural stability, could be improved by employing organic-cation-free MHPs in optoelectronic devices such as solar cells and light-emitting devices (LEDs). Due to their enticing features, including spectral tunability over the entire visible spectrum with high color purity, all-inorganic perovskites have become a focus of intense research for LEDs. This Review explores and discusses the application of all-inorganic CsPbX3 nanocrystals (NCs) in developing blue and white LEDs. We discuss the challenges perovskite-based LEDs (PLEDs) face and the potential strategies adopted to establish state-of-the-art synthetic routes to obtain rational control over dimensions and shape symmetry without compromising the optoelectronic properties. Finally, we emphasize the significance of matching the driving currents of different LED chips and balancing the aging and temperature of individual chips to realize efficient, uniform, and stable white electroluminescence.
Databáze: OpenAIRE