Long holographic lifetimes in bacteriorhodopsin films
Autor: | Daniel Tod Smithey, Marshall David Crew, Doǧan A. Timuçin, John D. Downie |
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Rok vydání: | 1998 |
Předmět: | |
Zdroj: | Optics Letters. 23:730 |
ISSN: | 1539-4794 0146-9592 |
DOI: | 10.1364/ol.23.000730 |
Popis: | The D85N genetic variant of bacteriorhodopsin displays a nearly permanent lifetime of the photochromic P490 state. We present pump-probe measurements that demonstrate this behavior. However, experimental diffraction efficiency measurements made from holograms recorded in a hydrated D85N film show markedly different decay behavior, suggesting a molecular diffusion process occurring in the film. Holograms recorded with different grating frequencies display correspondingly different decay times which support this hypothesis. A thin D85N film was then fabricated which was chemically crosslinked, resulting in the elimination of diffusion of BR molecules within the polymer matrix. This film exhibits a grating lifetime on the order of weeks or more, thus allowing the long term holographic storage of information in a BR film. |
Databáze: | OpenAIRE |
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