Long holographic lifetimes in bacteriorhodopsin films

Autor: Daniel Tod Smithey, Marshall David Crew, Doǧan A. Timuçin, John D. Downie
Rok vydání: 1998
Předmět:
Zdroj: Optics Letters. 23:730
ISSN: 1539-4794
0146-9592
DOI: 10.1364/ol.23.000730
Popis: The D85N genetic variant of bacteriorhodopsin displays a nearly permanent lifetime of the photochromic P490 state. We present pump-probe measurements that demonstrate this behavior. However, experimental diffraction efficiency measurements made from holograms recorded in a hydrated D85N film show markedly different decay behavior, suggesting a molecular diffusion process occurring in the film. Holograms recorded with different grating frequencies display correspondingly different decay times which support this hypothesis. A thin D85N film was then fabricated which was chemically crosslinked, resulting in the elimination of diffusion of BR molecules within the polymer matrix. This film exhibits a grating lifetime on the order of weeks or more, thus allowing the long term holographic storage of information in a BR film.
Databáze: OpenAIRE