European aerosol phenomenology − 8: Harmonised source apportionment of organic aerosol using 22 Year-long ACSM/AMS datasets
| Autor: | Gang Chen, Francesco Canonaco, Anna Tobler, Wenche Aas, Andres Alastuey, James Allan, Samira Atabakhsh, Minna Aurela, Urs Baltensperger, Aikaterini Bougiatioti, Joel F. De Brito, Darius Ceburnis, Benjamin Chazeau, Hasna Chebaicheb, Kaspar R. Daellenbach, Mikael Ehn, Imad El Haddad, Konstantinos Eleftheriadis, Olivier Favez, Harald Flentje, Anna Font, Kirsten Fossum, Evelyn Freney, Maria Gini, David C Green, Liine Heikkinen, Hartmut Herrmann, Athina-Cerise Kalogridis, Hannes Keernik, Radek Lhotka, Chunshui Lin, Chris Lunder, Marek Maasikmets, Manousos I. Manousakas, Nicolas Marchand, Cristina Marin, Luminita Marmureanu, Nikolaos Mihalopoulos, Griša Močnik, Jaroslaw Nęcki, Colin O'Dowd, Jurgita Ovadnevaite, Thomas Peter, Jean-Eudes Petit, Michael Pikridas, Stephen Matthew Platt, Petra Pokorná, Laurent Poulain, Max Priestman, Véronique Riffault, Matteo Rinaldi, Kazimierz Różański, Jaroslav Schwarz, Jean Sciare, Leïla Simon, Alicja Skiba, Jay G. Slowik, Yulia Sosedova, Iasonas Stavroulas, Katarzyna Styszko, Erik Teinemaa, Hilkka Timonen, Anja Tremper, Jeni Vasilescu, Marta Via, Petr Vodička, Alfred Wiedensohler, Olga Zografou, María Cruz Minguillón, André S.H. Prévôt |
|---|---|
| Přispěvatelé: | Paul Scherrer Institute (PSI), Datalystica, Norwegian Institute for Air Research (NILU), Centre d'Investigació i Desenvolupament [Barcelona] (CID-CSIC), Consejo Superior de Investigaciones Científicas [Madrid] (CSIC), University of Manchester [Manchester], Leibniz Institute for Tropospheric Research (TROPOS), Finnish Meteorological Institute (FMI), National Observatory of Athens (NOA), Ecole nationale supérieure Mines-Télécom Lille Douai (IMT Nord Europe), Institut Mines-Télécom [Paris] (IMT), Martin Ryan Institute, National University of Ireland [Galway] (NUI Galway), Laboratoire Chimie de l'environnement (LCE), Aix Marseille Université (AMU)-Institut de Chimie du CNRS (INC)-Centre National de la Recherche Scientifique (CNRS), Institut National de l'Environnement Industriel et des Risques (INERIS), Institute for Atmospheric and Earth System Research (INAR), Helsingin yliopisto = Helsingfors universitet = University of Helsinki, National Center for Scientific Research 'Demokritos' (NCSR), Meteorologisches Observatorium Hohenpeißenberg (MOHp), Deutscher Wetterdienst [Offenbach] (DWD), Imperial College London, Laboratoire de Météorologie Physique (LaMP), Institut national des sciences de l'Univers (INSU - CNRS)-Centre National de la Recherche Scientifique (CNRS)-Université Clermont Auvergne (UCA), Tallinn University of Technology (TTÜ), Czech Academy of Sciences [Prague] (CAS), Estonian Environmental Research Center, Tallinn, Estonia, National Institute of Research and Development for Optoelectronics (INOE), University Politehnica of Bucharest [Romania] (UPB), Jozef Stefan Institute [Ljubljana] (IJS), University of Nova Gorica, AGH University of Science and Technology [Krakow, PL] (AGH UST), Department of Environmental Systems Science [ETH Zürich] (D-USYS), Eidgenössische Technische Hochschule - Swiss Federal Institute of Technology [Zürich] (ETH Zürich), Laboratoire des Sciences du Climat et de l'Environnement [Gif-sur-Yvette] (LSCE), Université de Versailles Saint-Quentin-en-Yvelines (UVSQ)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Institut national des sciences de l'Univers (INSU - CNRS)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS), Climate and Atmosphere Research Centre (CARE-C), The Cyprus Institute, Nicosia, 2121, Cyprus, Istituto di Scienze dell'Atmosfera e del Clima [Bologna] (ISAC), National Research Council of Italy | Consiglio Nazionale delle Ricerche (CNR), Faculty of Physics and Applied Computer Science [Kraków] (FPACS), Aix Marseille Université (AMU), Estonian Environmental Research Centre (EKUK), Consejo Superior de Investigaciones Científicas [Spain] (CSIC), ANR-11-LABX-0005,Cappa,Physiques et Chimie de l'Environnement Atmosphérique(2011), European Project: 689443,H2020,H2020-SC5-2015-one-stage,ERA-PLANET(2016), European Project: 262254,EC:FP7:INFRA,FP7-INFRASTRUCTURES-2010-1,ACTRIS(2011), European Project: 654109,H2020,H2020-INFRAIA-2014-2015,ACTRIS-2(2015), European Project: 638703,H2020,ERC-2014-STG,COALA(2015), Natural Environment Research Council (NERC), European Commission, Ilmatieteen laitos, Finnish Meteorological Institute |
| Jazyk: | angličtina |
| Předmět: |
Source apportionment
spektrometrit FOS: Physical sciences European overview Harmonised protocol Organic aerosol Long-term datasets Rolling PMF pienhiukkaset Organic Aerosol fine particles 114 Physical sciences poltto polttoturve fuel peat kiinteät polttoaineet combustion (active) atmosphere (earth) Harmonised Protocol [SDU.ENVI]Sciences of the Universe [physics]/Continental interfaces environment General Environmental Science aerosolit ilmakehä [SDU.OCEAN]Sciences of the Universe [physics]/Ocean Atmosphere spectrometers European Overview emissions Long-term Datasets air quality Physics - Atmospheric and Oceanic Physics [SDU]Sciences of the Universe [physics] ilmanlaatu Atmospheric and Oceanic Physics (physics.ao-ph) [SDE]Environmental Sciences päästöt solid fuels aerosols Environmental Sciences |
| Zdroj: | Environment International Environment International, 2022, 166, pp.107325. ⟨10.1016/j.envint.2022.107325⟩ COLOSSAL ACSM collaboration 2022, ' European aerosol phenomenology − 8 : Harmonised source apportionment of organic aerosol using 22 Year-long ACSM/AMS datasets ', Environment International, vol. 166, 107325 . https://doi.org/10.1016/j.envint.2022.107325 Environment International, 166 Digital.CSIC. Repositorio Institucional del CSIC instname Environment international |
| ISSN: | 0160-4120 1873-6750 |
| DOI: | 10.1016/j.envint.2022.107325 |
| Popis: | Organic aerosol (OA) is a key component of total submicron particulate matter (PM1), and comprehensive knowledge of OA sources across Europe is crucial to mitigate PM1 levels. Europe has a well-established air quality research infrastructure from which yearlong datasets using 21 aerosol chemical speciation monitors (ACSMs) and 1 aerosol mass spectrometer (AMS) were gathered during 2013–2019. It includes 9 non-urban and 13 urban sites. This study developed a state-of-the-art source apportionment protocol to analyse long-term OA mass spectrum data by applying the most advanced source apportionment strategies (i.e., rolling PMF, ME-2, and bootstrap). This harmonised protocol was followed strictly for all 22 datasets, making the source apportionment results more comparable. In addition, it enables quantification of the most common OA components such as hydrocarbon-like OA (HOA), biomass burning OA (BBOA), cooking-like OA (COA), more oxidised-oxygenated OA (MO-OOA), and less oxidised-oxygenated OA (LO-OOA). Other components such as coal combustion OA (CCOA), solid fuel OA (SFOA: mainly mixture of coal and peat combustion), cigarette smoke OA (CSOA), sea salt (mostly inorganic but part of the OA mass spectrum), coffee OA, and ship industry OA could also be separated at a few specific sites. Oxygenated OA (OOA) components make up most of the submicron OA mass (average = 71.1%, range from 43.7 to 100%). Solid fuel combustion-related OA components (i.e., BBOA, CCOA, and SFOA) are still considerable with in total 16.0% yearly contribution to the OA, yet mainly during winter months (21.4%). Overall, this comprehensive protocol works effectively across all sites governed by different sources and generates robust and consistent source apportionment results. Our work presents a comprehensive overview of OA sources in Europe with a unique combination of high time resolution (30–240 min) and long-term data coverage (9–36 months), providing essential information to improve/validate air quality, health impact, and climate models. Environment International, 166 ISSN:0160-4120 ISSN:1873-6750 |
| Databáze: | OpenAIRE |
| Externí odkaz: |
|