Real-Time Observation of Charge-Spin Cooperative Dynamics Driven by a Nonequilibrium Phonon Environment

Autor: Kazuyuki Kuroyama, Sadashige Matsuo, Jo Muramoto, Shunsuke Yabunaka, Sascha R. Valentin, Arne Ludwig, Andreas D. Wieck, Yasuhiro Tokura, Seigo Tarucha
Rok vydání: 2022
Předmět:
Zdroj: Physical Review Letters. 129
ISSN: 1079-7114
0031-9007
DOI: 10.1103/physrevlett.129.095901
Popis: Quantum dots are recognized as a suitable platform for studying thermodynamic phenomena involving single electronic charges and spins in nano-scale devices. However, such a thermodynamic system is usually driven by electron reservoirs at different temperatures, not by a lattice temperature gradient. We report on experimental observations of charge-spin cooperative dynamics in transitions of two-electron spin states in a GaAs double quantum dot located in a non-equilibrium phonon environment. Enhancements in the spin-flip processes are observed, originating from phonon excitation combined with the spin-orbit interaction. In addition, due to the spatial gradient of phonon density between the dots, the spin-flip rate during an inter-dot electron tunnel from a hot to a cold dot is more enhanced than in the other direction, resulting in accumulation of parallel spin states in the double dot.
Databáze: OpenAIRE