Multi-particle momentum correlations extracted using covariance methods on multiple-ionization of diiodomethane molecules by soft-X-ray free-electron laser pulses
| Autor: | Makina Yabashi, Kiyonobu Nagaya, Kensuke Tono, Ahmad Nemer, Marko Huttula, Eetu Pelimanni, Shu Saito, Tsukasa Takanashi, Yu Luo, Thomas Gaumnitz, Shigeki Owada, Marta Berholts, Daehyun You, Akinobu Niozu, Minna Patanen, Per Johnsson, Shin-ichi Wada, Hironobu Fukuzawa, Hanna Myllynen, Edwin Kukk, Naomichi Yokono, Kiyoshi Ueda, Naoki Kishimoto |
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| Rok vydání: | 2020 |
| Předmět: |
Physics
Coulomb explosion General Physics and Astronomy 02 engineering and technology Covariance 021001 nanoscience & nanotechnology 01 natural sciences Molecular physics Ion Momentum chemistry.chemical_compound chemistry Ionization 0103 physical sciences Femtosecond Physics::Atomic and Molecular Clusters Diiodomethane Physical and Theoretical Chemistry 010306 general physics 0210 nano-technology Spectroscopy |
| Zdroj: | Physical Chemistry Chemical Physics. 22:2648-2659 |
| ISSN: | 1463-9084 1463-9076 |
| DOI: | 10.1039/c9cp03638e |
| Popis: | Momenta of ions from diiodomethane molecules after multiple ionization by soft-X-ray free-electron-laser pulses are measured. Correlations between the ion momenta are extracted by covariance methods formulated for the use in multiparticle momentum-resolved ion time-of-flight spectroscopy. Femtosecond dynamics of the dissociating multiply charged diiodomethane cations is discussed and interpreted by using simulations based on a classical Coulomb explosion model including charge evolution. |
| Databáze: | OpenAIRE |
| Externí odkaz: |
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