Multi-particle momentum correlations extracted using covariance methods on multiple-ionization of diiodomethane molecules by soft-X-ray free-electron laser pulses

Autor: Makina Yabashi, Kiyonobu Nagaya, Kensuke Tono, Ahmad Nemer, Marko Huttula, Eetu Pelimanni, Shu Saito, Tsukasa Takanashi, Yu Luo, Thomas Gaumnitz, Shigeki Owada, Marta Berholts, Daehyun You, Akinobu Niozu, Minna Patanen, Per Johnsson, Shin-ichi Wada, Hironobu Fukuzawa, Hanna Myllynen, Edwin Kukk, Naomichi Yokono, Kiyoshi Ueda, Naoki Kishimoto
Rok vydání: 2020
Předmět:
Zdroj: Physical Chemistry Chemical Physics. 22:2648-2659
ISSN: 1463-9084
1463-9076
Popis: Momenta of ions from diiodomethane molecules after multiple ionization by soft-X-ray free-electron-laser pulses are measured. Correlations between the ion momenta are extracted by covariance methods formulated for the use in multiparticle momentum-resolved ion time-of-flight spectroscopy. Femtosecond dynamics of the dissociating multiply charged diiodomethane cations is discussed and interpreted by using simulations based on a classical Coulomb explosion model including charge evolution.
Databáze: OpenAIRE