High-Curie-temperature ferromagnetism in self-organized Ge1−xMnx nanocolumns

Autor: Pascale Bayle-Guillemaud, Romain Dujardin, Joel Cibert, Alain Marty, J. Rothman, Serge Tatarenko, Edith Bellet-Amalric, A. Barski, Matthieu Jamet, Richard Mattana, Thibaut Devillers, V. Poydenot
Rok vydání: 2006
Předmět:
Zdroj: Nature Materials. 5:653-659
ISSN: 1476-4660
1476-1122
DOI: 10.1038/nmat1686
Popis: The emerging field of spintronics would be dramatically boosted if room-temperature ferromagnetism could be added to semiconductor nanostructures that are compatible with silicon technology. Here, we report a high-TC (>400 K) ferromagnetic phase of (Ge,Mn) epitaxial layer. The manganese content is 6%, and careful structural and chemical analyses show that the Mn distribution is strongly inhomogeneous: we observe eutectoid growth of well-defined Mn-rich nanocolumns surrounded by a Mn-poor matrix. The average diameter of these nanocolumns is 3 nm and their spacing is 10nm. Their composition is close to Ge2Mn, which corresponds to an unknown germanium-rich phase, and they have a uniaxially elongated diamond structure. Their Curie temperature is higher than 400 K. Magnetotransport reveals a pronounced anomalous Hall effect up to room temperature. A giant positive magnetoresistance is measured from 7,000% at 30K to 200% at 300K and 9 T, with no evidence of saturation.
Databáze: OpenAIRE