Modeling the time-dependent electron dynamics in dielectric materials induced by two-color femtosecond laser pulses: Applications to material modifications

Autor: E. O. Smetanina, Guillaume Duchateau, B. Chimier, P. González de Alaiza Martínez, Illia Thiele
Přispěvatelé: Centre d'Etudes Lasers Intenses et Applications (CELIA), Centre National de la Recherche Scientifique (CNRS)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université de Bordeaux (UB), Université de Bordeaux (UB)-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Centre National de la Recherche Scientifique (CNRS)
Jazyk: angličtina
Rok vydání: 2021
Předmět:
Zdroj: Physical Review A
Physical Review A, American Physical Society 2021, 103 (3), ⟨10.1103/PhysRevA.103.033107⟩
Physical Review A, 2021, 103 (3), ⟨10.1103/PhysRevA.103.033107⟩
ISSN: 2469-9926
2469-9934
DOI: 10.1103/PhysRevA.103.033107⟩
Popis: Controlling the electron dynamics during laser-matter interactions is a key factor to control the energy deposition and subsequent material modifications induced by femtosecond laser pulses. One way to achieve this goal is to use two-color femtosecond laser pulses. In this paper, the electron dynamics in dielectric materials induced by two-color femtosecond laser pulses is studied by solving dedicated optical Bloch equations. This model includes photo- and impact ionization, the laser heating of conduction electrons, their recombination to the valence band, and their collisions with phonons. The influence of photon energies, laser intensities, and pulse-to-pulse delay is analyzed. Depending on the interaction process, colors cooperate to excite electrons or drive them independently. For the given laser parameters, an optimal pulse-to-pulse delay is found which enhances significantly the energy deposition into the material, in agreement with experimental observations.
Databáze: OpenAIRE