Angularly resolved photoionization dynamics in atoms and molecules combining temporally and spectrally resolved experiments at ATTOLab and Synchrotron SOLEIL

Autor: Jennifer Joseph, Fabian Holzmeier, David Bresteau, Thierry Ruchon, Jean-Christophe Houver, Robert R. Lucchese, Danielle Dowek
Přispěvatelé: Institut des Sciences Moléculaires d'Orsay (ISMO), Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS), Attophysique (ATTO), Institut Rayonnement Matière de Saclay (IRAMIS), Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université Paris-Saclay-Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université Paris-Saclay-Laboratoire Interactions, Dynamiques et Lasers (ex SPAM) (LIDyl), Commissariat à l'énergie atomique et aux énergies alternatives (CEA)-Université Paris-Saclay-Centre National de la Recherche Scientifique (CNRS)-Centre National de la Recherche Scientifique (CNRS), Lawrence Berkeley National Laboratory [Berkeley] (LBNL), ANR-10-LABX-0039,PALM,Physics: Atoms, Light, Matter(2010), ANR-11-EQPX-0005,ATTOLAB,Plateforme pour la dynamique attoseconde(2011), European Project: 674960,H2020,H2020-MSCA-ITN-2015,ASPIRE(2016), European Project: 871124
Jazyk: angličtina
Rok vydání: 2023
Předmět:
Zdroj: The European Physical Journal. Special Topics
The European Physical Journal. Special Topics, 2023, ⟨10.1140/epjs/s11734-023-00815-7⟩
ISSN: 1951-6355
1951-6401
DOI: 10.1140/epjs/s11734-023-00815-7⟩
Popis: International audience; We report results for XUV-IR two-photon ionization of Ar, Ne, NO, and O2, where an XUV attosecond pulse train is superimposed with a synchronized IR pulse, obtained at the ATTOLab laser facility using electron–ion coincidence 3D momentum spectroscopy. Temporally resolved photoelectron angular distributions providing angle-resolved time-delays for np ionization of Ar and Ne, achieved by reconstruction of attosecond beating by interference of two-photon transitions through a unified formalism (Joseph et al. in J Phys B At Mol Opt Phys 53:184007, 2020), are summarized. For inner valence XUV-IR dissociative photoionization of NO and O2 molecules, we report electron–ion kinetic energy correlation diagrams and disentangle the dissociative photoionization processes relying on parallel XUV experiments at Synchrotron SOLEIL. For ionization into the NO+(c3Π) ionic state, extending the formalism developed for single-photon ionization, we focus on photoelectron angular distributions averaged on the delay between the XUV and the IR field in the field frame, molecular frame, and electron frame of reference.
Databáze: OpenAIRE
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