ZSM-5-confined Cr1–O4 active sites boost methane direct oxidation to C1 oxygenates under mild conditions
Autor: | Mengyu Zeng, Lu Cheng, Qingqing Gu, Bing Yang, Baiyang Yu, Jing Xu, Ying Zhang, Chengsi Pan, Xiao-Ming Cao, Yang Lou, Yongfa Zhu |
---|---|
Rok vydání: | 2023 |
Zdroj: | EES Catalysis. 1:153-161 |
ISSN: | 2753-801X |
Popis: | Cr1–O4 as an active site in the Cr1/ZSM-5 SAC can catalyze the DOM to form value-added C1 oxygenated products with a productivity of 21 100 μmol gcat−1 h−1 and a selectivity of 99.8% at 50 °C within 30 min, which outperforms most state-of-the-art catalysts. |
Databáze: | OpenAIRE |
Externí odkaz: |