Many-photon excitation of spherically symmetric molecules in an infrared laser field by weakly forbidden ΔR≠0, Δn≠0 vibrational–rotational transitions
Autor: | I N Knyazev, V V Lobko |
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Rok vydání: | 1980 |
Předmět: | |
Zdroj: | Soviet Journal of Quantum Electronics. 10:154-162 |
ISSN: | 0049-1748 |
DOI: | 10.1070/qe1980v010n02abeh009913 |
Popis: | An analysis is made of a model of multistage excitation of triply degenerate vibrations of spherically symmetric molecules in a strong infrared laser field. This involves allowing for weakly forbidden ?R?0, ?n?0 transitions. It is shown that as a result of these transitions, a system of up to several dozen multistage resonances is established within the absorption band. These resonances cover a group of rotational levels with different values of J (up to 10?20 values) and ensure that a considerable proportion of the molecules is excited to high vibrational states (up to ? = 10?15). |
Databáze: | OpenAIRE |
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