Integrated Experimental–Technoeconomic Analysis of the Lifetime of Pd–Au Membranes
| Autor: | Liang-Chih Ma, Yi Hua Ma, Nikolaos Kazantzis, Bernardo Castro-Dominguez, Ivan P. Mardilovich |
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| Rok vydání: | 2016 |
| Předmět: |
Materials science
Hydrogen General Chemical Engineering Alloy Composite number chemistry.chemical_element Nanotechnology 02 engineering and technology General Chemistry Permeance engineering.material 010402 general chemistry 021001 nanoscience & nanotechnology 01 natural sciences Industrial and Manufacturing Engineering 0104 chemical sciences Characterization (materials science) Membrane chemistry Chemical engineering engineering Chemical stability 0210 nano-technology Palladium |
| Zdroj: | Industrial & Engineering Chemistry Research. 55:10160-10171 |
| ISSN: | 1520-5045 0888-5885 |
| DOI: | 10.1021/acs.iecr.6b01898 |
| Popis: | Palladium and palladium/alloy membranes have shown to be an effective technology option for the production of pure hydrogen. In particular, Pd/Au membranes have displayed superior chemical stability and separation performance. However, the lack of industrial operating experience gives rise to technological uncertainties such as the lifetime of the membranes which could potentially prevent the deployment of this new technology option. In light of the above recognition, the primary aim of the present research work is to combine long-term H2 membrane permeance and He leak characterization tests (cumulative testing over 2.2 years) conducted to estimate the lifetime of composite asymmetric Pd/Au membranes at different thicknesses with a comprehensive economic performance assessment framework in the presence of inherent trade-offs between permeance, thickness, and membrane lifetime. The experimental results are depicted in terms of the produced H2 purity and flux at different testing times and various membrane ... |
| Databáze: | OpenAIRE |
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