A Comparison Study of the Effects of Ba and La Doping in Sr2IrO4: Ir–O–Ir Bond Angle and Carrier Concentration

Autor: Lei Luo, Yongjian Wang, Changjin Zhang, Jixiang Gong, Hui Han, Yuheng Zhang, D. D. Liang, Tao Han, Jing-Rong Wang, W. K. Zhu, Jun Yang
Rok vydání: 2017
Předmět:
Zdroj: Journal of Superconductivity and Novel Magnetism. 30:3493-3496
ISSN: 1557-1947
1557-1939
DOI: 10.1007/s10948-017-4152-z
Popis: We perform a systematic investigation on the effects of Ba and La doping on the lattice and transport properties of Sr2IrO4, which is theoretically predicted to be a host compound of high-temperature superconductivity. We observe a drastic straightening of the Ir–O–Ir bond angle in the Ba-doped samples. The straightening of the bond angle is much weaker in the La-doped samples. It is found that the La doping leads to the introduction of electron-type charge carriers, while the charge carrier concentration does not change too much in the Ba-doped samples. As a result, both the resistivity and the magnetic moments decrease much faster in the La-doped samples, compared to those in the Ba-doped samples. The present results suggest that it is the charge carrier density rather than the Ir–O–Ir bond angle that dominates the magnetic and transport properties of the Sr2IrO4 system.
Databáze: OpenAIRE