Magnetic Properties in the Normal State of LuNi2B2C Observed by61Ni and11B NMR
Autor: | W. F. Peck, Hidenori Takagi, J. J. Krajewski, Akira Ohno, Hiroshi Yasuoka, Robert J. Cava, Kenji Ikushima |
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Rok vydání: | 1997 |
Předmět: | |
Zdroj: | Journal of the Physical Society of Japan. 66:1130-1137 |
ISSN: | 1347-4073 0031-9015 |
Popis: | The 61 Ni spin-lattice relaxation rate, 6l Ti 1 -1 , and the Knight shift of a 91% 61 Ni enriched sample of LuNi 2 B 2 C have been measured in the normal state. It was found that 61 (T 1 T) -1 shows a Curie-Weiss like behavior, while the Knight shift has a slight temperature dependence. The hyperfine coupling constant is estimated to be 61 A = -16 kOe/μ B , which is an order of magnitude smaller than that due to the 3d-core-polarization mechanism. When the orbital term of the relaxation rate is given by the formula calculated for the tetragonal (D 2d ) symmetry at the 61 Ni sites, much larger d-spin term than that expected from the Knight shift is obtained. The Korringa relation is also discussed on the assumption that the hyperfine coupling constant is reduced by a strong s-d admixture, and then the deviation from the Korringa relation for free electrons, K(α), is more than one. This result suggests the significance of the generalized susceptibility, X(q), at finite wave vectors. |
Databáze: | OpenAIRE |
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