Efficient ambient ammonia synthesis by Lewis acid pair over cobalt single atom catalyst with suppressed proton reduction

Autor: Ngoc Quang Tran, Xinghui Liu, Yunhee Cho, Le Thai Duy, Lirong Zheng, Jianmin Yu, Sara Ajmal, Xiaodong Shao, Jinsun Lee, Hyoyoung Lee
Rok vydání: 2022
Předmět:
Zdroj: Journal of Materials Chemistry A. 10:8432-8439
ISSN: 2050-7496
2050-7488
DOI: 10.1039/d2ta00308b
Popis: A Lewis acid pair over a single Co atom anchored on sponge-like nitrogen-doped mesoporous hollow carbon nanofibers was designed. The catalyst exhibits an NH3 production rate of 67.6 μg h−1 mg−1 and a maximum Faraday efficiency of 56.9% at a peak potential of −0.1 V vs. RHE.
Databáze: OpenAIRE