Interrelation of the magnetic structure and the band insulating state in doped manganites

Autor: V. V. Deriglazov, S. M. Dunaevsky
Rok vydání: 2010
Předmět:
Zdroj: Physics of the Solid State. 52:904-906
ISSN: 1090-6460
1063-7834
Popis: The interrelation between the magnetic structure and the band insulating state in doped La1 − xCaxMnO3 manganites has been discussed. An analysis of various zigzag chains has revealed that, in the one-dimensional spectrum of eg electrons of these compounds, there always appear a number of band gaps, which at certain electron concentrations x support the formation of an insulating state in the corresponding three-dimensional antiferromagnetic structures. Apart from the well-known spectra of chains of the type (1 × 1) (magnetic E-structure) and (2 × 2) (magnetic CE-structure), we have obtained for the first time the spectrum of a (3 × 3) zigzag chain, whose three-dimensional unit cell contains 24 manganese atoms and provides a qualitatively correct fit to the magnetic structure of the La1/3Ca2/3MnO3 manganite. As follows from our analysis, the formation of a magnetic structure in this manganite should also be accompanied by the generation of a spontaneous magnetic moment.
Databáze: OpenAIRE