Single Semiconductor Nanostructure Extinction Spectroscopy
Autor: | Masaru Kuno, Ilia M. Pavlovetc, Rusha Chatterjee, Kyle Aleshire |
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Rok vydání: | 2018 |
Předmět: |
Heterodyne
Nanostructure Materials science business.industry Semiconductor nanostructures 02 engineering and technology Photothermal therapy 010402 general chemistry 021001 nanoscience & nanotechnology 01 natural sciences Ray 0104 chemical sciences Surfaces Coatings and Films Electronic Optical and Magnetic Materials General Energy Extinction (optical mineralogy) Modula Optoelectronics Physical and Theoretical Chemistry 0210 nano-technology business Spectroscopy |
Zdroj: | The Journal of Physical Chemistry C. 122:16443-16463 |
ISSN: | 1932-7455 1932-7447 |
Popis: | While emission-based, single-particle microscopies and spectroscopies have been highly successful in revealing the properties of matter hidden by ensemble averages, their limits have now become apparent. To address recognized future needs and, in particular, the need to go beyond fluorescent specimens, single-particle extinction techniques have been developed. Motivating this has been the desire to acquire information about the electronic structure of nanoscale materials difficult to obtain otherwise using either ensemble or emission-based, single-particle measurements. These techniques are, however, nontrivial since single nanostructures attenuate only 0.0001–1% of the incident light. This Review Article describes the challenges associated with overcoming the low signal-to-noise ratios inherent to low-dimensional semiconductor nanostructure extinction measurements. It simultaneously describes the fundamental operating principles and achievements of photothermal heterodyne imaging (PHI) and spatial modula... |
Databáze: | OpenAIRE |
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