Spin wave excitations in the pyrovanadate α−Cu2V2O7

Autor: Indra Dasgupta, Helen Walker, Sayantika Bhowal, Amitava Bhattacharyya, D. T. Adroja, Subham Majumdar, J. Sannigrahi, Asok K. Banerjee
Rok vydání: 2016
Předmět:
Zdroj: Physical Review B. 94
ISSN: 2469-9969
2469-9950
DOI: 10.1103/physrevb.94.144426
Popis: The pyrovanadate $\ensuremath{\alpha}\ensuremath{-}{\mathrm{Cu}}_{2}{\mathrm{V}}_{2}{\mathrm{O}}_{7}$ belongs to the orthorhombic ($Fdd2$) class of crystals with noncentrosymmetric crystal structure. Recently, the compound has been identified to be a magnetic multiferroic with a substantial electric polarization below the magnetic transition temperature ${T}_{C}$ = 35 K. Here we report the results of our inelastic neutron-scattering (INS) studies on a polycrystalline sample of $\ensuremath{\alpha}\ensuremath{-}{\mathrm{Cu}}_{2}{\mathrm{V}}_{2}{\mathrm{O}}_{7}$. Our INS data clearly show the existence of dispersive spin wave excitations below ${T}_{C}$ with a zone-boundary energy of 11 meV at 5 K. We have analyzed the data using linear spin wave theory, which shows good agreement between the experiment and calculation. The analysis is consistent with the third-nearest-neighbor exchange interaction playing a dominant role in the magnetism of the material.
Databáze: OpenAIRE