The effect of angular-momentum alignment on light-induced drift in gaseous mixtures

Autor: G Nienhuis, J J M Beenakker, I Kuscer
Rok vydání: 1994
Předmět:
Zdroj: Journal of Physics B: Atomic, Molecular and Optical Physics. 27:1361-1370
ISSN: 1361-6455
0953-4075
DOI: 10.1088/0953-4075/27/7/011
Popis: Theories of light-induced drift in gaseous mixtures have so far disregarded the alignment of angular momentum produced in optical excitation. The error caused thereby is estimated in terms of a first-order perturbation in non-sphericity of the intermolecular interaction. For transitions with Delta J=0 the result is not likely to exceed the order of 1% of the unperturbed drift velocity, which is below the experimental error margin. On the other hand, for Delta J=+or-1 and small J, a much larger influence for the alignment must be expected. The formalism also leads to an estimate for the precession effect caused by a magnetic field. In case of Sigma to Pi excitations of diamagnetic diatomic molecules this effect may become relatively strong.
Databáze: OpenAIRE