Determination of the 14C Content in Activated Steel Components from a Neutron Spallation Source and a Nuclear Power Plant

Autor: Benjamin Volmert, Ines Günther-Leopold, Tanja Stowasser, Erich Wieland, Dorothea Schumann, H.P. Linder
Rok vydání: 2014
Předmět:
Zdroj: Analytical Chemistry. 86:5448-5454
ISSN: 1520-6882
0003-2700
DOI: 10.1021/ac500654a
Popis: The (14)C content in activated steel components from the Swiss Nuclear Power Plant (NPP) Gosgen and the Spallation Neutron Source SINQ at the Paul Scherrer Institute is determined using a wet chemistry digestion technique and liquid scintillation counting for (14)C activity measurements. The (14)C activity of an activated fuel assembly steel nut from the NPP is further compared with theoretical predictions made on the basis of a Monte Carlo reactor model for this NPP. Knowledge of the (14)C inventory in these activated steel materials is important in conjunction with future corrosion studies on these materials aimed at identifying the (14)C containing organic compounds possibly formed in the cement-based near field of a repository for radioactive waste.
Databáze: OpenAIRE